Volume 9 Issue 6
Nov.  2019
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SUN Yixin, CAO Gang, DAI Jingfu, ZHANG Chunyu, SHEN Zhiqiang, SONG Yudong, HE Xuwen, ZHOU Yuexi. A cleaning method for anion exchange membrane fouled by sodium polyacrylate[J]. Journal of Environmental Engineering Technology, 2019, 9(6): 666-672. doi: 10.12153/j.issn.1674-991X.2019.04.040
Citation: SUN Yixin, CAO Gang, DAI Jingfu, ZHANG Chunyu, SHEN Zhiqiang, SONG Yudong, HE Xuwen, ZHOU Yuexi. A cleaning method for anion exchange membrane fouled by sodium polyacrylate[J]. Journal of Environmental Engineering Technology, 2019, 9(6): 666-672. doi: 10.12153/j.issn.1674-991X.2019.04.040

A cleaning method for anion exchange membrane fouled by sodium polyacrylate

doi: 10.12153/j.issn.1674-991X.2019.04.040
  • Received Date: 2019-02-25
  • Publish Date: 2019-11-20
  • Anion exchange membrane fouling caused by sodium polyacrylate (PAS) is one of the critical factors that affect organic acid recovery from butyl acrylate wastewater through bipolar membrane electrodialysis. To address this problem, a cleaning method for PAS-fouled anion exchange membrane was developed. The cleaning efficiency of PAS-fouled membrane was evaluated by analysis of membrane resistance, transference number and X-ray photo-electronic spectroscopy (XPS). The cleaning performances with three different cleaning solutions (sodium hydroxide, sodium chloride, and hydrochloric acid) and ultrasonic enhanced cleaning indicated that hydrochloric acid had the best cleaning performance, and the ultrasound could enhance the cleaning effect of all the three solutions. The membrane resistance and transference number of the fouled anion exchange membrane could almost be restored to the same level as uncontaminated membrane when using ultrasound-enhanced cleaning process with 2.0 mol/L hydrochloric acid as cleaning solution.

     

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  • [1]
    范志庆, 宋玉栋, 周岳溪 . 离子色谱法测定丙烯酸丁酯生产废水中丙烯酸和对甲基苯磺酸[J]. 中国环境监测, 2010,26(3):26-29.

    FAN Z Q, SONG Y D, ZHOU Y X . Determination of acrylic acid and p-toluenesulfonic acid in butyl acrylate-production wastewater by ion chromatography[J]. Environmental Monitoring in China, 2010,26(3):26-29.
    [2]
    王百党, 宋玉栋, 程家运 , 等. 丙烯酸盐及对甲苯磺酸盐对乙酸、丙酸产甲烷活性的影响[J]. 环境工程技术学报, 2014,4(5):393-398.
    doi: 10.3969/j.issn.1674-991X.2014.05.063

    WANG B D, SONG Y D, CHENG J Y , et al. Influence of acrylate and p-toluenesulfonate on methane-producing activity with acetic acid or propionic acid as substrate[J]. Journal of Environmental Engineering Technology, 2014,4(5):393-398. doi: 10.3969/j.issn.1674-991X.2014.05.063
    [3]
    余丽娜, 宋玉栋, 周岳溪 , 等. 电催化还原技术处理丙烯酸盐废水的研究[J]. 环境科学, 2011,32(10):2956-2960.

    YU L N, SONG Y D, ZHOU Y X , et al. Treatment of acrylate wastewater by electrocatalytic reduction process[J]. Environmental Science, 2011,32(10):2956-2960.
    [4]
    李鑫, 宋玉栋, 周岳溪 , 等. 双极膜电渗析法回收丙烯酸丁酯废水中的有机酸[J]. 化工环保, 2011,31(3):197-201.

    LI X, SONG Y D, ZHOU Y X , et al. Recovery of organic acid from butyl acrylate wastewater by bipolar membrane electrodialysis process[J]. Environmental Protection of Chemical Industry, 2011,31(3):197-201.
    [5]
    胡田, 宋玉栋, 周岳溪 , 等. 操作电压对双极膜电渗析回收丙烯酸丁酯废水中有机酸的影响[J]. 环境工程技术学报, 2014,4(6):456-461.
    doi: 10.3969/j.issn.1674-991X.2014.06.072

    HU T, SONG Y D, ZHOU Y X , et al. Effect of operating voltage on organic acid recovery from butyl-acrylate wastewater with bipolar membrane electrodialysis[J]. Journal of Environmental Engineering Technology, 2014,4(6):456-461. doi: 10.3969/j.issn.1674-991X.2014.06.072
    [6]
    宋玉栋, 曹刚, 徐守强 , 等. 光谱分析法鉴别丙烯酸丁酯废水中的阴离子交换膜污染物[J]. 光谱学与光谱分析, 2017,37(9):2832-2837.

    SONG Y D, CAO G, XU S Q , et al. Spectral analysis for the identification of anion exchange membrane pollutants in butyl-acrylate wastewater[J]. Spectroscopy and Spectral Analysis, 2017,37(9):2832-2837.
    [7]
    MONDOR M, IPPERSIEL D, LAMARCHE F , et al. Fouling characterization of electrodialysis membranes used for the recovery and concentration of ammonia from swine manure[J]. Bioresource Technology, 2009,100(2):566-571.
    [8]
    SCARAZZATO T, PANOSSIAN Z, TENORIO J A S,et al. Water reclamation and chemicals recovery from a novel cyanide-free copper plating bath using electrodialysis membrane process[J]. Desalination, 2018,436:114-124.
    [9]
    MIKHAYLIN S, BAZINET L . Fouling on ion-exchange membranes:classification, characterization and strategies of prevention and control[J]. Advances in Colloid and Interface Science, 2016,229:34-56.
    [10]
    CHOI M J, CHAE K J, AJAYI F F , et al. Effects of biofouling on ion transport through cation exchange membranes and microbial fuel cell performance[J]. Bioresource Technology, 2011,102:298-303.
    [11]
    LEE S, SHON H K, HONG S . Dewatering of activated sludge by forward osmosis (FO) with ultrasound for fouling control[J]. Desalination, 2017,421:79-88.
    [12]
    LUJAN-FACUNDO M J, MENDOZA-ROCA J A, CUARTAS-URIB B , et al. Membrane fouling in whey processing and subsequent cleaning with ultrasounds for a more sustainable process[J]. Journal of Cleaner Production, 2017,143:804-813.
    [13]
    SPETTMANN D, EPPMANN S, FLEMMING H C , et al. Visualization of membrane cleaning using confocal laser scanning microscopy[J]. Desalination, 2008,224:195-200.
    [14]
    PARVIZIAN F, RAHIMI M, HOSSEINI S M , et al. The effect of high frequency ultrasound on diffusion boundary layer resistance in ion-exchange membrane transport[J]. Desalination, 2012,286:155-165.
    [15]
    QASIM M, DARWISH N N, MHIYO S , et al. The use of ultrasound to mitigate membrane fouling in desalination and water treatment[J]. Desalination, 2018,443:143-164.
    [16]
    曹连城 . 离子交换膜选择透过性的测定[J]. 武汉化工学院学报, 1999,21(2):30-33.

    CAO L C . The test of ion exchange membrane selective permeability[J]. Journal of Wuhan Institute of Chemical Technology, 1999,21(2):30-33.
    [17]
    张维润 . 电渗析工程学[M]. 北京: 科学出版社, 1995.
    [18]
    BACHER L E, OLIVEIRA C, GIACOBBO A , et al. Coupling coagulation using tannin-based product with electrodialysis reversal to water treatment: a case study[J]. Journal of Environmental Chemical Engineering, 2017,5:6008-6015.
    [19]
    MASKOOKI A, KOBAYASHI T, MORTAZAVI S A , et al. Effect of low frequencies and mixed wave of ultrasound and EDTA on flux recovery and cleaning of microfiltration membranes[J]. Separation and Purification Technology, 2018,59(1):67-73.
    [20]
    MUTHUKUMARAN S, YANG K, SEUREN A , et al. The use of ultrasonic cleaning for ultrafiltration membranes in the dairy industry[J]. Separation and Purification Technology, 2004,39(1/2):99-107.
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