Volume 11 Issue 2
Mar.  2021
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LI Mingzhu, XU Jun, LIU Houfeng, GONG Anbao, DU Xiaohui. PM2.5 source apportionment over Jinan Metropolitan Area[J]. Journal of Environmental Engineering Technology, 2021, 11(2): 209-216. doi: 10.12153/j.issn.1674-991X.20200145
Citation: LI Mingzhu, XU Jun, LIU Houfeng, GONG Anbao, DU Xiaohui. PM2.5 source apportionment over Jinan Metropolitan Area[J]. Journal of Environmental Engineering Technology, 2021, 11(2): 209-216. doi: 10.12153/j.issn.1674-991X.20200145

PM2.5 source apportionment over Jinan Metropolitan Area

doi: 10.12153/j.issn.1674-991X.20200145
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  • Corresponding author: XU Jun E-mail: xujun@craes.org.cn
  • Received Date: 2020-06-09
  • Publish Date: 2021-03-20
  • Based on the PSAT particulate source tracing technology of camx model, the quantitative analysis of PM2.5 pollution, regional transport law and sector contribution for cities over Jinan Metropolitan Area were performed for year 2016. The results showed that in terms of the annual mean source apportionment of PM2.5, for the local area of Jinan City, the emission accounted for about 50%, while the whole Jinan Metropolitan Area contributed 75%. The mutual contributions among Jinan Metropolitan Area cities were obvious, up to 13%. In summer, the local contribution was the largest and the regional transport in the eastern Shandong region had the highest impact on the study area by 24%. While in winter, affected by the winter monsoon, the regional transport from Beijing-Tianjin-Hebei Region increased, up to 24%. At present, as far as Jinan Metropolitan Area was concerned, the major sectors contributed to PM2.5 included industrial boilers, steel industry, fugitive dust, chemical industry, metallurgical industry, building material industry, and automobile source. The targeted counter-measure for the above sectors may be a fast and effective approach to reduce PM2.5 pollution.

     

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  • [1]
    WANG L L, WU G F, GAUTAM A, et al. Spatio-temporal variation characteristics of PM2.5 in the Beijing-Tianjin-Hebei Region,China,from 2013 to 2018[J]. Environmental Research and Public Health, 2019,16(21):4276.
    [2]
    王彤, 华阳, 许庆成, 等. 京津冀郊区站点秋冬季大气PM2.5来源解析[J]. 环境科学, 2019,40(3):1035-1042.

    WANG T, HUA Y, XU Q C, et al. Source apportionment of PM2.5 in suburban area of Beijing-Tianjin-Hebei Region in autumn and winter[J]. Environmental Science, 2019,40(3):1035-1042.
    [3]
    刘旭艳. 京津冀PM2.5区域传输模拟研究[D]. 北京:清华大学, 2015:13-15.
    [4]
    温新欣, 崔兆杰, 张桂芹. 济南市PM2.5来源的解析[J]. 济南大学学报(自然科学版), 2009,23(3):292-295.

    WEN X X, CUI Z J, ZHANG G Q. Analysis of the source apportionment of PM2.5 in Jinan[J]. Journal of University of Jinan(Science and Technology), 2009,23(3):292-295.
    [5]
    刘雨思, 李杏茹, 张怡萌, 等. 济南市秋冬季大气细粒子污染特征及来源[J]. 环境化学, 2017,36(4):787-798.

    LIU Y S, LI X R, ZHANG Y M, et al. Characteristics and sources of airborne fine particles during the fall and winter in Jinan[J]. Environmental Chemistry, 2017,36(4):787-798.
    [6]
    孙友敏, 李少洛, 陈春竹, 等. 济南市机动车排气污染特征及对市区PM2.5的影响[J]. 环境科学学报, 2018,38(4):1384-1391.

    SUN Y M, LI S L, CHEN C Z, et al. Study on characteristics of vehicle exhaust and the influence on PM2.5 in Jinan City[J]. Acta Scientiae Circumstantiae, 2018,38(4):1384-1391.
    [7]
    杨佳美, 刘保双, 毕晓辉, 等. 泰安市环境受体PM2.5组分特征与来源解析[J]. 环境科学与技术, 2017,40(9):153-160.

    YANG J M, LIU B S, BI X H, et al. Chemical composition characteristics and source apportionment of ambient PM2.5 in Tai’an[J]. Environmental Science and Technology, 2017,40(9):153-160.
    [8]
    ZHANG Y, SHEN J, LI Y. An atmospheric vulnerability assessment framework for environment management and protection based on CAMx[J]. Journal of Environmental Management, 2018,207:341-354.
    pmid: 29182979
    [9]
    GOLIFF W S, STOCKWELL W R. The regional atmospheric chemistry mechanism,version 2[J]. Atmospheric Environment, 2013,68:174-185.
    [10]
    HODZIC A, AUMONT B, KNOTE C, et al. Volatility dependence of Henry’s law constants of condensable organics:application to estimate depositional loss of secondary organic aerosols[J]. Geophysical Research Letters, 2014,41:4795-4804.
    [11]
    KNOTE C, HODZIC A, JMENEZ J L. The effect of dry and wet deposition of condensable vapors on secondary organic aerosols concentrations over the continental US[J]. Atmospheric Chemistry and Physics, 2015,15:1-18.
    [12]
    薛文博, 付飞, 王金南, 等. 中国PM2.5跨区域传输特征数值模拟研究[J]. 中国环境科学, 2014,34(6):1361-1368.

    XUE W B, FU F, WANG J N, et al. Numerical study on the characteristics of regional transport of PM2.5 in China[J]. China Environmental Science, 2014,34(6):1361-1368.
    [13]
    陈云波, 徐峻, 何友江, 等. 北京市冬季典型重污染时段PM2.5污染来源模式解析[J]. 环境科学研究, 2016,29(5):627-636.

    CHEN Y B, XU J, HE Y J, et al. Model analytic research of typical heavy PM2.5 pollution periods in winter in Beijing[J]. Research of Environmental Sciences, 2016,29(5):627-636.
    [14]
    WANG Y J, BAO S W, WANG S X, et al. Local and reginal contributions to fine particulate matter in Beijing during heavy haze episodes[J]. Science of the Total Environment, 2017,580:283-296.
    [15]
    US Environmental Protection Agency. User’s guide comprehensive air quality model with extensions Version 6.40[R]. Novato California:Ramboll Environ, 2016:6-28.
    [16]
    杜晓惠, 徐峻, 刘厚凤, 等. 重污染天气下电力行业排放对京津冀地区PM2.5的贡献[J]. 环境科学研究, 2016,29(4):475-482.

    DU X H, XU J, LIU H F, et al. Contribution of power plant emissions to PM2.5 over Beijing-Tianjin-Hebei Area during heavy pollution periods[J]. Research of Environmental Sciences, 2016,29(4):475-482.
    [17]
    曹国良, 张小曳, 龚山陵, 等. 中国区域主要颗粒物及污染气体的排放源清单[J]. 科学通报, 2011,56(3):261-268.

    CAO G L, ZHANG X Y, GONG S L, et al. Emission inventories of primary particles and pollutant gases for China[J]. Chinese Science Bulletin, 2011,56(3):261-268.
    [18]
    ZHANG Q, STREETS D G, CARMICHAEL G R, et al. Asian emissions in 2006 for the NASA INTEX-B mission[J]. Atmospheric Chemistry and Physics, 2009,173:5131-5153.
    [19]
    OHARA T, AKIMOTO H, KUROKAWA J, et al. An Asian emission inventory of anthropogenic emission sources for the period 1980-2020[J]. Atmospheric Chemistry and Physics, 2007,7(100):4419-4444.
    [20]
    ZHAO B, WANG P, MA J Z, et al. A high-resolution emission inventory of primary pollutants for the Huabei Region,China[J]. Atmospheric Chemistry and Physics, 2012,12:481-501.
    [21]
    “2+26”城市大气污染源排放清单研究[R]. 北京:中国环境科学研究院, 2019.
    [22]
    GUENTHER A, KARL T, HARLEY P, et al. Estimates of global terrestrial isoprene emissions using MEGAN(Model of Emissions of Gases and Aerosols from Nature)[J]. Atmospheric Chemistry and Physics, 2006,6(68):3181-3210
    [23]
    GUENTHER A, HEALD C L, DUHL T, et al. The model of emissions of gases and aerosols from nature version 2.1(MEGAN 2.1):an extended and updated framework for modeling biogenic emissions[J]. Atmospheric Chemistry and Physics, 2006,68:1471-1492.
    [24]
    BOVE M C, BROTIO P, CASSOLA F, et al. An integrated PM2.5 source apportionment study:positive matrix factorisation vs.the chemical transport model CAMx[J]. Atmospheric Environment, 2014,94:274-286.
    [25]
    徐峻, 杜晓惠, 马圣冉, 等. 重污染应急控制措施效果的快速评估方法[J]. 环境工程, 2018,36(4):165-169.

    XU J, DU X H, MA S R, et al. Quick assessment method of effects of countermeasures in response to severe air pollution[J]. Environmental Engineering, 2018,36(4):165-169.
    [26]
    薛亦峰, 闫静, 宋光武, 等. 大气污染物排放清单的建立及不确定性[J]. 城市环境与城市生态, 2012(2):31-33.

    XUE Y F, YAN J, SONG G W, et al. Establishment of an air pollutant emission inventory and uncertainty analysis[J]. Urban Environment & Urban Ecology, 2012(2):31-33.
    [27]
    BOYLAN J W, RUSSELL A G. PM and light extinction model performance metrics,goals,and criteria for three-dimensional air quality model[J]. Atmospheric Environment, 2006,40(26):4946-4959.
    [28]
    贾海鹰, 程念亮, 何友江, 等. 2014年春季山东省PM2.5跨界输送研究[J]. 环境科学, 2015,36(7):2353-2360.

    JIA H Y, CHENG N L, HE Y J, et al. Numerical study on the characteristics of regional transport of PM2.5 in Shandong Province during spring in 2014[J]. Environmental Science, 2015,36(7):2353-2360.
    [29]
    王庆, 刘诗军. 影响山东夏季降水的季风水汽输送特征分析[J]. 气象科学, 2006(2):197-202.

    WANG Q, LIU S J. The correlative analysis between moisture transport over monsoon areas and the summer rainfall in Shandong Province[J]. Journal of the Meteorological Sciences, 2006(2):197-202.
    [30]
    庞海洋, 孔祥生, 贺正洋, 等. 山东半岛降雪时空分布特征[J]. 地球信息科学学报, 2019,21(11):1721-1734.

    PANG H Y, KONG X S, HE Z Y, et al. Spatiotemporal distribution of the snowfall in Shandong Peninsula[J]. Journal of Geo-Information Science, 2019,21(11):1721-1734.
    [31]
    WANG X Y, DICKINSON R E, SU L Y, et al. PM2.5 pollution in China and how it has been exacerbated by terrain and meteorological conditions[J]. Bulletin of the American Meteorological Society, 2018,99(1):105-119.
    [32]
    刘新玲, 王晓明, 李小明. 2000—2004年山东中西部五城市大气污染变化特征[J]. 科学技术与工程, 2008(12):3390-3396.

    LIU X L, WANG X M, LI X M. Analysis on variation characteristics of air pollution in five cities in central and western Shandong Province during 2000-2004[J]. Science Technology and Engineering, 2008(12):3390-3396.
    [33]
    彭玏, 赵媛媛, 赵吉麟, 等. 京津冀大气污染传输通道区大气污染时空格局研究[J]. 中国环境科学, 2019,39(2):449-458.

    PENG L, ZHAO Y Y, ZHAO J L, et al. Spatiotemporal patterns of air pollution in air pollution transmission channel of Beijng-Tian-Hebei from 2000 to 2015[J]. China Environmental Science, 2019,39(2):449-458.
    [34]
    LIU B S, SONG N, DAI Q L, et al. Chemical composition and source apportionment of ambient PM2.5 during the non-heating period in Taian,China[J]. Atmospheric Research, 2016,170:23-33.
    [35]
    LIN M Y, OKI T, BENGTSSON M, et al. Long-range transport of acidifying substances in East Asia:PartⅡ.source-receptor relationships[J]. Atmospheric Environment, 2008,42(24):5956-5967.
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