Volume 11 Issue 3
May  2021
Turn off MathJax
Article Contents
Article Navigation >  Journal of Environmental Engineering Technology  > 2021  >  11(3): 459-467
ZHU Yunjie, ZHU Xiaoyan, LIN Yingzi, XU Qiujin. Screening of priority pollutants in Liaodong Bay[J]. Journal of Environmental Engineering Technology, 2021, 11(3): 459-467. doi: 10.12153/j.issn.1674-991X.20200222
Citation: ZHU Yunjie, ZHU Xiaoyan, LIN Yingzi, XU Qiujin. Screening of priority pollutants in Liaodong Bay[J]. Journal of Environmental Engineering Technology, 2021, 11(3): 459-467. doi: 10.12153/j.issn.1674-991X.20200222
shu

Screening of priority pollutants in Liaodong Bay

doi: 10.12153/j.issn.1674-991X.20200222
  • 1.

    School of Municipaland Environmental Engineering, Jilin Jianzhu University

  • 2.

    Center for Global Health, Nanjing Medical University

  • 3.

    Chinese Research Academy of Environmental Sciences

More Information
  • Corresponding author: ZHU Xiaoyan E-mail: zhuxy0613@126.com; LIN Yingzi E-mail: linyingzi1000@163.com
  • Received Date: 2020-09-14
  • Publish Date: 2021-05-20
    Abstract
  • Liaodong Bay is an important coastal economic zone in China and has carried a large number of pollutants discharged from coastal areas for many years. Heavy metal and organic pollution are serious in coastal waters. The composite scoring method and potential risk index method were used to screen the priority pollutants based on the 12 pollutants of water quality monitoring data in the coastal waters of Liaodong Bay in 2016-2018. The results showed that the total score of the 12 pollutants using the composite scoring method was 29.4-83.2. There were three types of class Ⅰ pollutants, including Hg (83.2), Cd (83.2) and Pb (75.8), and there were three categories of class Ⅱ pollutants, namely Cu (68.4), Cr (63.2) and As (60.8). The results of potential risk index method ranged from 4 to 22. There were three types of class Ⅰ pollutants, including Cd (22), Cu (20) and As (20), and there were three categories of class Ⅱ pollutants, including Hg (19), Cr (19) and Pb (19). Combining the two grading methods, considering that the common primary pollutant screened by the two methods was Cu and the average detected concentrations of Hg, Pb, Cr, As and Cu in Liaodong Bay was 0.04, 2, 7.1, 1.8, 3.8 μg/L, respectively, while the corresponding water quality criterion continuous concentration recommended by US EPA was 0.94, 5.6, 50, 36, 3.1 μg/L, respectively, only Cu exceeded the water quality criterion continuous concentration. At the same time, the average concentration of Cu (3.8 μg/L) in Liaodong Bay was much higher than the set value of harmful concentration (1.90 μg/L) that protected 95% aquatic species. Therefore, Cd and Cu were proposed to be included in the list of priority pollutants for control in Liaodong Bay.

     

    • FullText(HTML)
  • loading
    • References(58)
  • [1]
    赖翔宇, 王世存. 中国近岸海域污染严重[J]. 生态经济, 2019, 35(3):9-12.
    [2]
    TANABE S, PRUDENTE M S, et al. Mussel watch: marine pollution monitoring in Asian waters[J]. Ocean & Coastal Management, 2000, 43(8/9):819-839.
    [3]
    BELLAS J, ALBENTOSA M, VIDAL-LIÑÁN L, et al. Combined use of chemical,biochemical and physiological variables in mussels for the assessment of marine pollution along the N-NW Spanish coast[J]. Marine Environmental Research, 2014, 96:105-117.
    doi: 10.1016/j.marenvres.2013.09.015
    [4]
    GADE M, ALPERS W. Using ERS-2 SAR images for routine observation of marine pollution in European coastal waters[J]. Science of the Total Environment, 1999, 237/238:441-448.
    doi: 10.1016/S0048-9697(99)00156-4
    [5]
    MONTEVECCHI W, FIFIELD D, BURKE C, et al. Tracking long-distance migration to assess marine pollution impact[J]. Biology Letters, 2012, 8(2):218-221.
    doi: 10.1098/rsbl.2011.0880
    [6]
    KUCUKSEZGIN F, KONTAS A, ALTAY O, et al. Assessment of marine pollution in Izmir Bay:nutrient,heavy metal and total hydrocarbon concentrations[J]. Environment International, 2006, 32(1):41-51.
    doi: 10.1016/j.envint.2005.04.007
    [7]
    ATSDR. ATSDR’s substance priority list[R/OL].(2020-01-17)[2020-09-05]. https://www.atsdr.cdc.gov/spl/.
    [8]
    SANDS P, GALIZZI P. Directive 2000/60/EC of the European Parliament and of the Council of 23 October 2000 establishing a framework for Community action in the field of water policy (OJ L 327 22.12.2000 p.1)[M]// Documents in European Community Environmental Law. Cambridge: Cambridge University Press: 879-969.
    [9]
    TEIXIDÓ E, TERRADO M, GINEBREDA A, et al. Quality assessment of river waters using risk indexes for substances and sites,based on the COMMPS procedure[J]. Journal of Environmental Monitoring, 2010, 12(11):2120-2127.
    doi: 10.1039/c0em00108b
    [10]
    DUNN A M. A relative risk ranking of selected substances on Canada’s national pollutant release inventory[J]. Human and Ecological Risk Assessment:an International Journal, 2009, 15(3):579-603.
    doi: 10.1080/10807030902892562
    [11]
    RAHA D, RICHARDS T. National pollutant inventory report for a water utility:a case study[C]// National Environment Conference. Queensland: Queensland Chapter,Environmental Engineering Society, 2003:384-389.
    [12]
    LERCHE D, MATSUZAKI S Y, SØRENSEN P B, et al. Ranking of chemical substances based on the Japanese Pollutant Release and Transfer Register using partial order theory and random linear extensions[J]. Chemosphere, 2004, 55(7):1005-1025.
    doi: 10.1016/j.chemosphere.2004.01.023
    [13]
    US EPA. Toxic and priority pollutants under the Clean Water Act:EPA 40 CFR Part 423,Appendix A[A/OL].(2014-01-19) [2020-04-03]. https://www.epa.gov/eg/toxic-and-priority-pollutants-under-clean-water-act.
    [14]
    US EPA. Risk assessment guidance for superfund:volume Ⅱ.environmental evaluation manual,interim final[A]. Washington DC: Office of Emergency and Remedial Response,US EPA, 1991.
    [15]
    US EPA. Risk-assessment guidance for superfund:volume Ⅰ.human health evaluation manual[A]. Washington DC: Office of Emergency and Remedial Response,US EPA, 1989.
    [16]
    US EPA Technical background document to support rule making pursuant to CERCLA section 102:volume 3[A]. Washington DC: Office of Solid Waste and Emergency Response,US EPA, 1989.
    [17]
    US EPA. Toxic chemical release inventory risk screening guide:version 1.0[A]. Washington DC: Office of Toxic Substances,US EPA, 1989.
    [18]
    裴淑玮, 周俊丽, 刘征涛. 环境优控污染物筛选研究进展[J]. 环境工程技术学报, 2013, 3(4):363-368.

    PEI S W, ZHOU J L, LIU Z T. Research progress on screening of environment priority pollutants[J]. Journal of Environmental Engineering Technology, 2013, 3(4):363-368.
    [19]
    周文敏, 傅德黔, 孙宗光. 中国水中优先控制污染物黑名单的确定[J]. 环境科学研究, 1991, 4(6):9-12.

    ZHOU W M, FU D Q, SUN Z G. Determination of black list of China’s priority pollutants in water[J]. Research of Environmental Sciences, 1991, 4(6):9-12.
    [20]
    傅德黔, 孙宗光, 周文敏. 中国水中优先控制污染物黑名单筛选程序[J]. 中国环境监测, 1990, 6(5):48-50.
    [21]
    中国环境优先监测研究课题组. 环境优先污染物[M]. 北京: 中国环境科学出版社, 1989.
    [22]
    胡冠九. 环境优先污染物简易筛选法初探[J]. 环境科学与管理, 2007, 32(9):47-49.

    HU G J. The primary screening method for environment priority pollutants[J]. Environmental Science and Management, 2007, 32(9):47-49.
    [23]
    李沫蕊, 王亚飞, 滕彦国, 等. 应用综合评分法筛选下辽河平原区域地下水典型污染物[J]. 北京师范大学学报(自然科学版), 2015, 51(1):64-68.

    LI M R, WANG Y F, TENG Y G, et al. Application of comprehensive evaluation for screening of typical pollutants in groundwater of the Liao River Basin[J]. Journal of Beijing Normal University (Natural Science), 2015, 51(1):64-68.
    [24]
    VOYSLAVOV T, TSAKOVSKI S, SIMEONOV V. Hasse diagram technique as a tool for water quality assessment[J]. Analytica Chimica Acta, 2013, 770:29-35.
    doi: 10.1016/j.aca.2013.01.063
    [25]
    刘存, 韩寒, 周雯, 等. 应用Hasse图解法筛选优先污染物[J]. 环境化学, 2003, 22(5):499-502.

    LIU C, HAN H, ZHOU W, et al. Applying hasse diagrams to select priority pollutants[J]. Environmental Chemistry, 2003, 22(5):499-502.
    [26]
    穆景利, 王菊英, 张志锋. 我国近岸海域优先控制有机污染物的筛选[J]. 海洋环境科学, 2011, 30(1):114-117.

    MU J L, WANG J Y, ZHANG Z F. Screening of priority-control organic pollutants in coastal water in China[J]. Marine Environmental Science, 2011, 30(1):114-117.
    [27]
    段一明, 张戈, 于大涛. 辽东湾西北部海域沉积物重金属含量分析及污染评价[J]. 海洋开发与管理, 2020, 37(1):39-45.

    DUAN Y M, ZHANG G, YU D T. Heavymetal content analysis and pollution evaluation in the northwest area of Liaodong Bay[J]. Ocean Development and Management, 2020, 37(1):39-45.
    [28]
    王萧, 张文思, 迟光希, 等. 辽东湾及其附近海域重金属污染研究进展[J]. 环境化学, 2019, 38(10):2317-2326.

    WANG X, ZHANG W S, CHI G X, et al. The heavy metals contamination in Liaodong Bay and its adjacent waters[J]. Environmental Chemistry, 2019, 38(10):2317-2326.
    [29]
    王焕松, 雷坤, 李子成, 等. 辽东湾北岸主要入海河流污染物入海通量及其影响因素分析[J]. 海洋学报, 2011, 33(6):110-116.

    WANG H S, LEI K, LI Z C, et al. Analysis of major pollutants flux into the sea and influencing factors on the north shore of the Liaodong Gulf[J]. Acta Oceanologica Sinica, 2011, 33(6):110-116.
    [30]
    吴金浩, 李强, 宋广军, 等. 2008—2017年夏季辽东湾北部渔业水域生态环境质量综合评价[J]. 生态与农村环境学报, 2019, 35(8):1000-1008.

    WU J H, LI Q, SONG G J, et al. Comprehensive assessment of eco-environmental quality of fishery waters in the northern Liaodong Bay in 2008-2017[J]. Journal of Ecology and Rural Environment,2019, 35(8):1000-1008.
    [31]
    方志刚, 穆云侠. 渤海辽东湾富营养化的趋势研究[J]. 环境保护科学, 2001, 27(3):15-17.

    FANG Z G, MU Y X. Research in the trend of eutrophication in Liaodung Bay of Bo Sea[J]. Environmental Protection Science, 2001, 27(3):15-17.
    [32]
    胡超魁, 李楠, 吴金浩, 等. 辽东湾近岸海域沉积物石油类分布特征及污染状况[J]. 海洋环境科学, 2020, 39(4):551-556.

    HU C K, LI N, WU J H, et al. Distribution character and pollution status of petroleum hydrocarbon in sediment in Liaodong Bay inshore sea areas[J]. Marine Environmental Science, 2020, 39(4):551-556.
    [33]
    李沫蕊, 王韦舒, 任姝娟, 等. 运用改进综合评分法筛选典型污染物的研究:以大武水源地地下水典型污染物筛选为例[J]. 环境污染与防治, 2014, 36(11):72-77.

    LI M R, WANG W S, REN S J, et al. Screening typical pollutants by modified comprehensive evaluation method:a case study of typical pollutants screening in groundwater of Dawu water source[J]. Environmental Pollution & Control, 2014, 36(11):72-77.
    [34]
    胡雷芳. 五种常用系统聚类分析方法及其比较[J]. 浙江统计, 2007(4):11-13.
    [35]
    宋利臣, 叶珍, 马云, 等. 潜在危害指数在水环境优先污染物筛选中的改进与应用[J]. 环境科学与管理, 2010, 35(9):20-22.

    SONG L C, YE Z, MA Y, et al. Theimprovement and application of potential damage index in screening priority pollutants in the water environment[J]. Environmental Science and Management, 2010, 35(9):20-22.
    [36]
    徐青. 饮用水源地优先控制污染物筛选研究[D]. 扬州: 扬州大学, 2015.
    [37]
    KINGSBURY G L, WHITE J B, WATSON J S. Multimedia environmental goals for environmental assessment:volume Ⅰ.supplement a.report for October 1978-October 1979[R]. North Carolina,US:Research Triangle Institute, 1980.
    [38]
    范薇, 周金龙, 曾妍妍, 等. 石河子地区地下水优先控制污染物的确定[J]. 人民黄河, 2018, 40(4):69-71.

    FAN W, ZHOU J L, ZENG Y Y, et al. Determination of priority control pollutants of groundwater in Shihezi area[J]. Yellow River, 2018, 40(4):69-71.
    [39]
    许秋瑾, 李丽, 梁存珍, 等. 淮安某县农村饮用水源中优控污染物的筛选研究[J]. 中国环境科学, 2013, 33(4):631-638.

    XU Q J, LI L, LIANG C Z, et al. Screening of priority control pollutants from the rural drinking water sources in Huai’an City[J]. China Environmental Science, 2013, 33(4):631-638.
    [40]
    胡望钧. 常见有毒化学品环境事故应急处置技术与监测方法[M]. 北京: 中国环境科学出版社, 1993.
    [41]
    王立阳, 李斌, 李佳熹, 等. 沈阳市典型城市河流优先控制污染物筛选及生态环境风险评估[J]. 环境科学研究, 2019, 32(1):25-34.

    WANG L Y, LI B, LI J X, et al. Priority pollutants and their ecological risk in typically urbanized river of Shenyang[J]. Research of Environmental Sciences, 2019, 32(1):25-34.
    [42]
    王莉, 王玉平, 卢迎红, 等. 辽河流域浑河沈阳段地表水重点控制有机污染物的筛选[J]. 中国环境监测, 2005, 21(6):59-62.

    WANG L, WANG Y P, LU Y H, et al. The sifting of priority control organic pollutants in Hunhe River of Liaohe Basin in Shenyang City[J]. Environmental Monitoring in China, 2005, 21(6):59-62.
    [43]
    洪鸣, 王菊英, 张志锋, 等. 海水中金属铅水质基准定值研究[J]. 中国环境科学, 2016, 36(2):626-633.

    HONG M, WANG J Y, ZHANG Z F, et al. Study on seawater quality criteria for lead[J]. China Environmental Science, 2016, 36(2):626-633.
    [44]
    王菊英, 穆景利, 王莹. 《海水水质标准(GB 3097—1997)》定值的合理性浅析:以铅和甲基对硫磷为例[J]. 生态毒理学报, 2015, 10(1):151-159.

    WANG J Y, MU J L, WANG Y. Rationality analysis of the existing marine water quality standard(GB 3097-1997):a case study on lead and methyl-parathion[J]. Asian Journal of Ecotoxicology,2015, 10(1):151-159.
    [45]
    周家义, 潜琬英, 刘敏光, 等. 海洋环境地球化学:Ⅰ.海水中铬的存在形态及其在海水—底质间相互交换研究[J]. 海洋与湖沼, 1980, 11(1):30-45.

    ZHOU J Y, QIAN W Y, LIU M G, et al. Marine environmental geochemistry:Ⅰ.the valency state of chromium in sea water and the sea-water-sediment chromium interchange[J]. Oceanologia et Limnologia Sinica, 1980, 11(1):30-45.
    [46]
    曲洪林, 刘东武. 铬对海洋生物的影响[J]. 生命科学仪器, 2008, 6(12):36-38.

    QU H L, LIU D W. The effects of chromium on marine biology[J]. Life Science Instruments, 2008, 6(12):36-38.
    [47]
    DONG Y, ROSENBAUM R K, HAUSCHILD M Z. Assessment of metal toxicity in marine ecosystems:comparative toxicity potentials for nine cationic metals in coastal seawater[J]. Environmental Science & Technology, 2016, 50(1):269-278.
    doi: 10.1021/acs.est.5b01625
    [48]
    康凯莉, 管博, 李正炎. 中国近海环境中汞的水质基准与生态风险[J]. 中国海洋大学学报(自然科学版), 2019, 49(1):102-114.

    KANG K L, GUAN B, LI Z Y. Marine water quality criteria derivation and ecological risk assessment for mercury in coastal waters in China[J]. Periodical of Ocean University of China, 2019, 49(1):102-114.
    [49]
    DURÁN I, BEIRAS R. Ecotoxicologically based marine acute water quality criteria for metals intended for protection of coastal areas[J]. Science of the Total Environment, 2013, 463/464:446-453.
    doi: 10.1016/j.scitotenv.2013.05.077
    [50]
    US EPA. National recommended water quality criteria:aquatic life criteria table[A/OL].(2019-10-10)[2020-08-29]. https://www.epa.gov/wqc/national-recommended-water-quality-criteria-aquatic-life-criteria-table#table.
    [51]
    辽宁省人民政府. 辽宁概况[EB/OL].[2020-09-02]. http://www.ln.gov.cn/zjln/lngk/.
    [52]
    陈丽芳. 矿山重金属污染研究现状及修复技术[J]. 中国金属通报, 2018(6):183-184.
    [53]
    金亚飚, 肖尚忠. 钢铁企业水环境污染防治措施探讨[J]. 给水排水, 2013, 49(9):60-62.
    [54]
    全燮, 孙英, 杨凤林, 等. 海域有机污染物优先排序和风险分类模糊评判系统[J]. 海洋环境科学, 1996, 15(1):1-7.

    QUAN X, SUN Y, YANG F L, et al. Fuzzy system for assessment of the prior order and the risk classification of the marine organic pollutants[J]. Marine Environmental Science, 1996, 15(1):1-7.
    [55]
    楼文高. 用密切值法进行海域有机污染物优先排序和风险分类研究[J]. 海洋环境科学, 2002, 21(3):43-48.

    LOU W G. Application of osculating method for the prior order and risk classification for the marine organic pollutants[J]. Marine Environmental Science, 2002, 21(3):43-48.
    [56]
    MAGGI C, ONORATI F, LAMBERTI C V, et al. The hazardous priority substances in Italy:national rules and environmental quality standard in marine environment[J]. Environmental Impact Assessment Review, 2008, 28(1):1-6.
    doi: 10.1016/j.eiar.2007.01.002
    [57]
    COMMISSION U E. Decision No. 2455/2001/EC of the European Parliament and of the Council establishing the list of priority substances in the field of water policy and amending Directive 2000/60/EC[J]. Official Journal of the European Union L 331, 2001:1-5.
    [58]
    WATERHOUSE J, BRODIE J. Identification of priority pollutants and priority areas in the Great Barrier Reef Catchments[R]. Keynes:Reef & Rainforest Research Centre, 2011.
    • Relative Articles
    • Supplements(0)
    • Cited By
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索
    Get Citation
    PDF
    XML

    Article Metrics

    Article Views(449) PDF Downloads(78) Cited by()
    Proportional views
    Related

    Copyright © Editorial Department of Journal of Environmental Engineering Technology

    京ICP备05031605号-2

    Supported by: Beijing Renhe Information Technology Co., Ltd.  

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return