Volume 7 Issue 3
May  2017
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Article Navigation >  Journal of Environmental Engineering Technology  > 2017  >  7(3): 268-277
WU Yafeng, CHEN Jianhua, ZHONG Lianhong, ZHANG Guoning. Emission characteristics and control status of fine particles emitted from coal-fired boilers[J]. Journal of Environmental Engineering Technology, 2017, 7(3): 268-277. doi: 10.3969/j.issn.1674-991X.2017.03.039
Citation: WU Yafeng, CHEN Jianhua, ZHONG Lianhong, ZHANG Guoning. Emission characteristics and control status of fine particles emitted from coal-fired boilers[J]. Journal of Environmental Engineering Technology, 2017, 7(3): 268-277. doi: 10.3969/j.issn.1674-991X.2017.03.039
shu

Emission characteristics and control status of fine particles emitted from coal-fired boilers

doi: 10.3969/j.issn.1674-991X.2017.03.039

  • 1. Research Institute of Environmental Standard, Chinese Research Academy of Environmental Sciences, Beijing 100012, China

  • 2. Beijing Municipal Research Institute of Environmental Protection, Beijing 100037, China

More Information
  • Corresponding author: CHEN Jianhua E-mail: chenjh@craes.org.com; ZHONG Lianhong E-mail: zhonglianhong@cee.cn
  • Received Date: 2016-10-31
  • Publish Date: 2017-05-20
    Abstract
  • Coal-fired boiler is one of the primary sources of ambient fine particulate matter in China in terms of source apportionment. In order to understand the emission characteristics and control status of fine particles emitted from coal-fired boilers, some relevant research findings both at home and abroad were summarized systematically, including the size distribution characteristics, component characteristics, emission forms and possible influencing factors of the fine particles. The removal efficiency of fine particles of current dedustors for the flue gas from coal-fired boilers as well as corresponding technical improvements on the dedustors was reviewed. Recent management situation of stationary pollution sources and sampling methods of fine particles both at home and abroad were summarized. Aiming at existing deficiency of research and management, several suggestions are proposed. Firstly, the research should be strengthen on the size distribution characteristics and formation mechanism of fine particles generated and emitted from coal-fired boilers from the point of view of source control, targeting the reduction of the emission of primary condensable particles and the precursors of secondary fine particles. Secondly, the study on component characteristics of fine particles from local coal-fired boilers should be strengthened. Thirdly, the development of efficient dedusting technologies should be accelerated, especially focusing on the affordable control technologies of fine particles for industrial coal-fired boilers. Fourthly, great attention should be paid to the study and management policy of the number concentration of fine particles and superfine particles. Finally, it is suggested that the standard sampling methods and emission limit of fine particles from stationary sources should be formulated by relevant administrative departments.

     

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    • References(70)
  • [1]
    环境保护部. 应急措施对空气污染加重趋势减缓有明显效果[EB/OL]. (2015-12-09)[2016-10-23]. http://www.mep.gov.cn/gkml/hbb/qt/201512/t20151209_318742.htm.
    [2]
    赵钦新, 王善武 . 我国工业锅炉未来发展分析[J]. 工业锅炉, 2007(1):1-9.
    [3]
    国家统计局. 废气中主要污染物排放年度数据[A/OL]. [2016-10-23]. http://data.stats.gov.cn/easyquery.htm?cn=C01.
    [4]
    环境保护部,国家发展和改革委员会,财政部. 重点区域大气污染防治“十二五”规划[A/OL]. [2016-10-23]. http://wenku.baidu.com/link?url=HdzNFvNWWdjqY0nEIOMFl44c0ThJPfO6aJVKykEYYI5Ttxe9mY6TiIzkBRKe5k2VNHCMU7UdqK_o884XLjdIk1dt5Gl7_15NdwWdDA2qK3W.
    [5]
    北京市环境保护局. 2014年北京市环境状况公报[A/OL]. [2016-12-23]. http://www.bjepb.gov.cn/bjepb/resource/cms/2015/04/2015041609380279715.pdf.
    [6]
    尹连庆, 殷春肖, 赵浩宁 , 等. 燃煤工业锅炉PM2.5排放规律[J]. 环境工程学报, 2014,8(5):2020-2024.

    YIN L Q, YIN C X, ZHAO H N , et al. Regular pattern of PM2.5 emission from coal-fired industrial boilers[J]. Chinese Journal of Environmental Engineering, 2014,8(5):2020-2024.
    [7]
    王书肖, 赵秀娟, 李兴华 , 等. 工业燃煤链条炉细粒子排放特征研究[J]. 环境科学, 2009,30(4):963-968.

    WANG S X, ZHAO X J, LI X H , et al. Emission characteristics of fine particles from grate firing boilers[J]. Environmental Science, 2009,30(4):963-968.
    [8]
    ZHAO Y, WANG S X, NIELSEN C P , et al. Establishment of a database of emission factors for atmospheric pollutants from Chinese coal-fired power plants[J]. Atmospheric Environment, 2010,44(12):1515-1523.
    [9]
    李超, 李兴华, 段雷 , 等. 燃煤工业锅炉可吸入颗粒物的排放特征[J]. 环境科学, 2009,30(3):650-655.

    LI C, LI X H, DUAN L , et al. Emission characteristics of PM10 coal-fired industrial boiler[J]. Environmental Science, 2009,30(3):650-655.
    [10]
    SEAMES W S . An initial study of the fine fragmentation fly ash particle mode generated during pulverized coal combustion[J]. Fuel Processing Technology, 2003,81(2):109-125.
    [11]
    LINAK W P, MILLER C A, SEAMES W S , et al. On trimodal particle size distributions in fly ash from pulverized-coal combustion[J]. Proceedings of the Combustion Institute, 2002,29(1):441-447.
    [12]
    EHRLICH C, NOLL G, KALKOFF W D , et al. PM10,PM2.5 and PM1.0:emissions from industrial plants:results from measurement programmes in Germany[J]. Atmospheric Environment, 2007,41(29):6236-6254.
    [13]
    CHENG R J, MOHNEN V A, SHEN T T , et al. Characterization of particulates from power plants[J]. Journal of the Air Pollution Control Association, 1976,26(8):787-790.
    [14]
    ZHANG C F, YAO Q, SUN J M . Characteristics of particulate matter from emissions of four typical coal-fired power plants in China[J]. Fuel Processing Technology, 2005,86(7):757-768.
    [15]
    MAMANE Y, MILLER J L, DZUBAY T G . Characterization of individual fly ash particles emitted from coal-and oil-fired power plants[J]. Atmospheric Environment, 1986,20(11):2125-2135.
    [16]
    NATUSCH D F S, WALLACE J R, EVANS C A . Toxic trace elements:preferential concentration in respirable particles[J]. Science, 1974,183:202-204.
    [17]
    KAAKINEN J W, JORDEN R M, LAWASANI M H , et al. Trace element behavior in coal-fired power plant[J]. Environmental Science & Technology, 1975,9:862-869.
    [18]
    GLADNEY E S, SMALL J A, GORDON G E , et al. Composition and size distribution of in-stack particulate material at a coal-fired power plant[J]. Atmospheric Environment, 1976,10(12):1071-1077.
    [19]
    段雷, 马子轸, 李振 , 等. 燃煤电厂排放细颗粒物的水溶性无机离子特征综述[J]. 环境科学, 2015,36(3):1117-1122.

    DUAN L, MA Z Z, LI Z , et al. Characteristics of water soluble inorganic ions in fine particles emitted from coal-fired power plants[J]. Environmental Science, 2015,36(3):1117-1122.
    [20]
    刘晓宇 . 典型固定燃烧源颗粒物排放特征研究[D]. 北京:中国环境科学研究院, 2007.
    [21]
    郭兴明, 郝吉明, 段雷 , 等. 大容量燃煤电站锅炉水溶性离子排放特征[J]. 清华大学学报(自然科学版), 2006,46(12):1991-1994.

    GUO X M, HAO J M, DUAN L , et al. Characteristics of water soluble ions from large coal-fired power plant boilers[J]. Journal of Tsinghua University (Science & Technology), 2006,46(12):1991-1994.
    [22]
    WANG H L, ZHENG P H, ZHANG Y H , et al. Characterization of inorganic components of size-segregated particles in the flue gas of a coal-fired power plant[J]. Energy & Fuels, 2008,22:1636-1640.
    [23]
    YAO X H, CHAN C K, FANG M , et al. The water-soluble ionic composition of PM2.5 in Shanghai and Beijing,China[J]. Atmosphere Environment, 2002,36(26):4223-4234.
    [24]
    耿彦红, 刘卫, 单健 , 等. 上海市大气颗粒物中水溶性离子的粒径分布特征[J]. 中国环境科学, 2010,30(12):1585-1589.

    GENG Y H, LIU W, SHAN J , et al. Characterization of major water-soluble ions sized-fractionated particulate matters in Shanghai[J]. China Environmental Science, 2010,30(12):1585-1589.
    [25]
    马召辉, 梁云平, 张健 , 等. 北京市典型排放源PM2.5成分谱研究[J]. 环境科学学报, 2015,35(12):4043-4052.

    MA Z H, LIANG Y P, ZHANG J , et al. PM2.5 profiles of typical sources in Beijing[J]. Acta Scientiae Circumstantiae, 2015,35(12):4043-4052.
    [26]
    史妍婷, 杜谦, 高建民 , 等. 燃煤锅炉PM2.5控制现状及改进建议[J]. 节能技术, 2013,31(4):345-348.

    SHI Y T, DU Q, GAO J M , et al. The PM2.5 control status of coal-fired boiler and improvable advice[J]. Energy Conservation Technology, 2013,31(4):345-348.
    [27]
    吕建燚, 李定凯 . 不同条件对煤粉燃烧后PM10、PM2.5、PM1.0排放影响的实验研究[J]. 中国电机工程学报, 2006,26(20):103-107.

    LÜ J Y, LI D K . Experimental study on PM10,PM2.5,PM1.0 emission features influenced by different conditions in pulverized coal combustion[J]. Proceeding of the CSEE, 2006,26(20):103-107.
    [28]
    张凯, 龚本根, 田冲 , 等. 燃煤细颗粒物排放实验及形成机理[J]. 煤炭学报, 2015,40(11):2696-2701.

    ZHANG K, GONG B G, TIAN C , et al. Formation mechanisms of fine particles generated from coal combustion[J]. Journal of China Coal Society, 2015,40(11):2696-2701.
    [29]
    TUCKER W G . An overview of PM2.5 sources and control strategies[J]. Fuel Processing Technology, 2000,65:379-392.
    [30]
    SHEN L H, WU J H, GAO Z P , et al. Characterization of chemical looping combustion of coal in a 1 kW the reactor with a nickel-based oxygen carrier[J]. Combustion and Flame, 2010,157(5):934-942.
    [31]
    贾明生, 凌长明 . 烟气酸露点温度的影响因素及其计算方法[J]. 工业锅炉, 2003(6):31-35.
    [32]
    超低排放还是煤改气、煤改生物质?燃煤锅炉该怎么治[EB/OL]. [2016-10-23]. http://mt.sohu.com/20160424/n445860179.shtml, 2016-04-24.
    [33]
    赵炬 . 工业锅炉除尘器的改进[J]. 机械管理开发, 2006(4):65-67.
    [34]
    王志轩, 张健宇, 潘磊 , 等. 中国电力减排研究:2013霾、PM2.5与火电厂细颗粒物控制[M]. 北京: 中国市场出版社, 2013.
    [35]
    代旭东, 徐晓亮, 缪明烽 . 电厂PM2.5排放现状与控制技术[J]. 能源环境保护, 2011,25(6):1-4.

    DAI X D, XU X L, MIAO M F . Emission status and control technology of ultra fire particles in coal-fired power plants[J]. Energy Environmental Protection, 2011,25(6):1-4.
    [36]
    贺晋瑜, 燕丽, 雷宇 , 等. 我国燃煤电厂颗粒物排放特征[J]. 环境科学研究, 2015,28(6):862-868.

    HE J Y, YAN L, LEI Y , et al. Emission characteristics of particulate matter from coal-fired power plants in China[J]. Research of Environmental Science, 2015,28(6):862-868.
    [37]
    YAO Q, LI S Q, XU H W , et al. Reprint of studies on formation and control of combustion particulate matter in China:a review[J]. Energy, 2010,35(11):4480-4493.
    [38]
    徐飞, 骆仲泱, 王鹏 , 等. 440 t/h循环流化床锅炉颗粒物排放特性的实验研究[J]. 中国电机工程学报, 2007,27(29):7-11.

    XU F, LUO Z Y, WANG P , et al. Experimental study on the characteristics of particulate matter emitted from a 440 t/h CFB coal-fired boiler[J]. Proceedings of the CSEE, 2007,27(29):7-11.
    [39]
    易红宏, 郝吉明, 段雷 , 等. 电厂除尘设施对PM10排放特征影响研究[J]. 环境科学, 2006,27(10):1921-1927.

    YI H H, HAO J M, DUAN L , et al. Influence of dust catchers on PM10 emission characteristics of power plants[J]. Environmental Science, 2006,27(10):1921-1927.
    [40]
    WU Z J, HU M, LIN P , et al. Particle number size distribution in the urban atmosphere of Beijing[J]. China, 2008,42(34):7967-7980.
    [41]
    KASPARIAN J, FREJAFON E, RAMBALDI P , et al. Characterization of urban aerosols using SEM-microscopy,X-ray analysis and Lidar measurements[J]. Atmospheric Environment, 1998,32(17):2957-2967.
    [42]
    郭欣, 陈丹, 郑楚光 , 等. 燃煤锅炉可吸入颗粒物排放规律研究[J]. 环境科学, 2008,29(3):587-592.

    GUO X, CHEN D, ZHENG C G , et al. Experimental study on emission characteristics of PM10 in coal-fired boilers[J]. Environmental Science, 2008,29(3):587-592.
    [43]
    杨传遍, 袁竹林, 杨林军 , 等. 袋式除尘器在国电九江电厂的应用及其对PM2.5的脱除分析[J]. 电力科技与环保, 2014,30(4):47-49.

    YANG C B, YUAN Z L, YANG L J , et al. Discussion on application of bag filter in Guodian Power Plant and its removal efficiency of PM2.5[J]. Electric Power Technology and Environmental Protection, 2014,30(4):47-49.
    [44]
    ZHAO Y, WANG S X, NIELSEN C P , et al. Establishment of a database of emission factors for atmospheric pollutants from Chinese coal-fired power plants[J]. Atmospheric Environment, 2010,44(12):1515-1523.
    [45]
    隋建才, 徐明厚, 丘纪华 , 等. 燃煤锅炉PM10形成与排放特性的实验研究[J]. 工程热物理学报, 2006,27(2):335-338.

    SUI J C, XU M H, QIU J H , et al. Formation and emission characteristics of PM10 at the coal-fired utility boiler[J]. Journal of Engineering Thermophysics, 2006,27(2):335-338.
    [46]
    王圣, 朱法华, 王慧敏 , 等. 基于实测的燃煤电厂细颗粒物排放特性分析与研究[J]. 环境科学学报, 2011,31(3):630-635.

    WANG S, ZHU F H, WANG H M , et al. Fine particle emission characteristics form coal-fired power plant based on field tests[J]. Acta Scientiae Circumstantiae, 2011,31(3):630-635.
    [47]
    尚伟, 黄超, 王菲 . 超细颗粒物PM2.5控制技术综述[J].环境科技, 2008(增刊2):75-78.
    [48]
    国家环境保护总局. 火电厂大气污染物排放标准:GB 13223—2011[S]. 北京: 中国环境科学出版社, 2011.
    [49]
    CHEN D, WU K, MI J . Experimental investigation of aerodynamic agglomeration of fine ash particles from a 330 MW PC-fired boiler[J]. Fuel, 2016,165:86-93.
    [50]
    王鹏, 骆仲泱, 徐飞 , 等. 复合式静电除尘器脱除电厂排放PM2.5研究[J]. 环境科学学报, 2007,27(11):1789-1792.

    WANG P, LUO Z Y, XU F , et al. PM2.5 removal from coal-fired power plant with combined ESP and pulse charge pretreatment[J]. Acta Scientiae Circumstantiae, 2007,27(11):1789-1792.
    [51]
    郝吉明, 段雷, 易红宏 , 等. 燃烧源可吸入颗粒物的物理化学特征[M]. 北京: 科学出版社, 2008.
    [52]
    王丽丽, 王丽萍, 张秀琨 , 等. 电袋复合式除尘器的工业化应用研究[J]. 电力环境保护, 2008,24(5):1-4.

    WANG L L, WANG L P, ZHANG X K , et al. Study on electro-bag compound dust removing technology in industrialization application[J]. Electric Power Environmental Protection, 2008,24(5):1-4.
    [53]
    朱继保 . 细颗粒物的电收集技术研究[D]. 杭州:浙江大学, 2010.
    [54]
    郭小玲, 唐晓飞, 赵海峰 , 等. 电袋复合式除尘器的发展趋势分析[J]. 华北电力技术, 2008(9):50-54.

    GUO X L, TANG X F, ZHAO H F , et al. Development trend of unified electric-bag composite dust-collector[J]. North China Electric Power, 2008(9):50-54.
    [55]
    NINOMIYA Y, WANG Q, XU S , et al. Effect of additives on the reduction of PM2.5 emissions during pulverized coal combustion[J]. Energy & Fuels, 2009,23(7):3412-3417.
    [56]
    环境保护部. 固定污染源排气中颗粒物测定与气态污染物采样方法:GB 16157—1996[S]. 北京: 中国环境科学出版社, 1996.
    [57]
    International Organization for Standardization. Stationary source emissions-determination of PM10/PM2.5 mass concentration in flue gas-measurement at low concentrations by use of impactors:ISO 23210: 2009[S/OL]. [2016-10-23]. http://www.iso.org/iso/home/store/catalogue_ics/catalogue_detail_ics.htm?ics1=13&ics2=40&ics3=40&csnumber=53379.
    [58]
    International Organization for Standardization. Stationary source emissions-test method for determining PM2.5 and PM10 mass in stack gases using cyclone samplers and sample dilution:ISO 25597: 2013[S/OL]. [2016-10-23]. http://www.iso.org/iso/iso_catalogue/catalogue_tc/catalogue_detail.htm?csnumber=43029.
    [59]
    环境保护部. 大气细颗粒物一次源排放清单编制技术指南[A/OL]. [2016-10-23]. http://www.mep.gov.cn/gkml/hbb/bgg/201408/W020140828351293619540.pdf.
    [60]
    环境保护部. 大气可吸入颗粒物一次源排放清单编制技术指南[A/OL]. [2016-10-23]. http://www.mep.gov.cn/gkml/hbb/bgg/201501/W020150107594587771088.pdf, 2014S.
    [61]
    蒋靖坤, 邓建国, 李振 , 等. 固定污染源排气中PM2.5采样方法综述[J]. 环境科学, 2014,35(5):2018-2024.

    JIANG J K, DENG J G, LI Z , et al. Sampling methods for PM2.5 from stationary sources:a review[J]. Environmental Science, 2014,35(5):2018-2024.
    [62]
    US EPA . Methods for measurement of filterable PM10 and PM2.5 and measurement of condensable particular matter emissions from stationary sources:Method 201A and 202[S/OL]. [2016-10-23]. http://www.thefederalregister.com/2010/12/21/2010-30847.html.
    [63]
    US EPA . Other test method 27(OTM 27)-determining PM10 and PM2.5 emissions from stationary sources[S/OL]. [2016-10-26]. https://www3.epa.gov/ttn/emc/prelim/otm27.pdf.
    [64]
    LU P, WU J, PAN W P . Particulate matter emissions from a coal-fired power plant[C]// Bioinformatics and biomedical engineering(ICBBE).Chengdu:2010 4th IEEE International Conference, 2010: 1-4.
    [65]
    US EPA . Other test method 28 (OTM 28):dry impinger method for determining condensable particulate emissions from stationary sources[S/OL]. [2016-10-26]. https://www3.epa.gov/ttn/emc/prelim/otm28.pdf.
    [66]
    周楠, 曾立民, 于雪娜 , 等. 固定源稀释通道的设计和外场测试研究[J]. 环境科学学报, 2006,26(5):764-772.

    ZHOU N, ZENG L M, YU X N , et al. The design and field test of a dilution tunnel for stationary sources[J]. 2006,26(5):764-772.
    [67]
    白志鹏, 朱坦, 葛苏 , 等. 2004烟道气稀释混合多通道分级采样器:ZL 03258297.8[P]. 2004-08-04.
    [68]
    李兴华, 段雷, 郝吉明 , 等. 固定燃烧源颗粒物稀释采样系统的研制与应用[J]. 环境科学学报, 2008,28(3):458-463.

    LI X H, DUAN L, HAO J M , et al. Design and application of a dilution stack sampling system for measuring particulate matter from stationary combustion sources[J]. Acta Scientiae Circumstantiae, 2008,28(3):458-463.
    [69]
    李兴华, 曹阳, 蒋靖坤 , 等. 固定源PM2.5稀释采样器的研制[J]. 环境科学学报, 2015,35(10):3309-3315.

    LI X H, CAO Y, JIANG J K , et al. Development of dilution sampler for measuring fine particle from stationary sources[J]. Acta Scientiae Circumstantiae, 2015,35(10):3309-3315.
    [70]
    International Organization for Standardization. Stationary source emissions-determination of PM10/PM2.5 mass concentration in flue gas-measurement at higher concentrations by use of virtual impactors:ISO 13271: 2012[S/OL]. [2016-10-23]. http://www.instrument.com.cn/download/StandardDetail_120980.htm.
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