Abstract:
Plutonium (Pu) is an important radionuclide that exists in the environment in trace or ultra-trace level, which is closely associated with the nuclear industry. The distribution characteristics, migration behavior and the application in geochemistry of
239+240Pu in soil and lake sediments in recent years in China were reviewed. The results showed that the sedimentation fluxes of
239+240Pu in soils were estimated at from 7.31 MBq/km
2 to 554.00 MBq/km
2; while that of
239+240Pu in lake sediments were from 4.80 MBq/km
2 to 240.60 MBq/km
2, varying with the environment and latitude in the study area.
240Pu/
239Pu isotope ratios from soils and lake sediments were found to be within 0.048-0.307 and 0.164-0.193, with an average of 0.181±0.026 and 0.179±0.021, respectively. Global atmospheric nuclear test sedimentation was the main source of
239+240Pu in China. As an important long-lived radionuclide, the combination of Pu isotope with other radionuclide tracing methods (e. g.
137Cs,
210Pb and
7Be tracing methods), remote sensing technology and traditional research methods should be strengthened in future research, which was conducive to improving the analysis accuracy of Pu in large-scale environmental areas and the tracing efficiency of
239+240Pu radionuclide tracing technology.