Characteristics and source analysis of water-soluble inorganic ions in PM2.5 in Yanqing District, Beijing
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摘要: 对2017年6月—2018年5月北京市延庆区大气PM2.5样本进行采集,分析了PM2.5中9种水溶性无机离子的污染特征,并利用SPSS软件进行来源解析。结果表明:延庆区大气PM2.5中总水溶性无机离子平均浓度为28.0 μg∕m 3,其中,SAbstract: The atmospheric PM2.5 samples were collected from June 2017 to May 2018 in Yanqing District, Beijing. The pollution characteristics of nine water-soluble inorganic ions in PM2.5 were analyzed, and the sources were analyzed by SPSS software. The results showed that the average concentration of total water-soluble inorganic ions in PM2.5 in Yanqing District was 28.0 μg∕m 3, of which S
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Key words:
- PM2.5 /
- water-soluble inorganic ions /
- source analysis
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[1] 胡敏 . 北京大气细粒子和超细粒子理化特征、来源及形成机制[M]. 北京:科学出版社 2009. [2] CHEN R, CHU C, TAN J , et al. Ambient air pollution and hospital admission in Shanghai,China[J]. Journal of Hazardous Materials, 2010,181(1∕2∕3):234-240. [3] World Bank . Cost of pollution in China:economic estimates of physical damages[M]. Washington DC:World Bank, 2007. [4] 古金霞, 吴丽萍, 霍光耀 , 等. 天津市PM2.5中水溶性无机离子污染特征及来源分析[J]. 中国环境监测, 2013,29(3):30-34.GU J X, WU L P, HUO G Y , et al. Pollution character and source of water-soluble inorganic ions in PM2.5 over Tianjin[J]. Environmental Monitoring in China, 2013,29(3):30-34. [5] YE B M, JI X L, YANG H Z , et al. Concentration and chemical composition of PM2.5 in Shanghai for all-yeat period[J]. Atmospheric Environment, 2003,37(4):499-510. [6] LIN J J . Characterization of the major chemical species in PM2.5 in the Kaohsiung City,Taiwan[J]. Atmospheric Environment, 2002,36(12):1911-1920. [7] 邱天雪, 陈进生, 尹丽倩 , 等. 闽南重点城市春季PM2.5中水溶性无机离子特征研究[J]. 生态环境学报, 2013,22(3):512-516.QIU T X, CHEN J S, YIN L Q , et al. Study on the characteristics of water-soluble inorganic ions in PM2.5 in spring in the key cities of southern Fujian Province[J]. Ecology and Environment Sciences, 2013,22(3):512-516. [8] WANG G H, WANG H, YU Y J , et al. Chemical characterization of water-soluble components of PM10 and PM2.5 atmospheric aerosols in five locations of Nanjing,China[J]. Atmospheric Environment, 2003,37(21):2893-2902. [9] YAO X H, CHAN C K, FANG M , et al. The water-soluble ionic composition of PM2.5 in Shanghai and Beijing,China[J]. Atmospheric Environment, 2002,36(26):4223-4234. [10] 赵晴 . 典型地区无机细粒子污染特征及成因研究[D]. 北京:清华大学, 2010. [11] 周敏, 陈长虹, 王红丽 , 等. 上海市秋季典型大气高污染过程中颗粒物的化学组成变化特征[J]. 环境科学学报, 2012,32(1):81-92.ZHOU M, CHEN C H, WANG H L , et al. Chemical characteristics of particulate matters during air pollution episodes in autumn of Shanghai,China[J]. Acta Scientiae Circumstantiae, 2012,32(1):81-92. [12] 杨懂艳, 刘保献, 张大伟 , 等. 2012—2013年间北京市PM2.5中水溶性离子时空分布规律及相关性分析[J]. 环境科学, 2015,36(3):768-773.YANG D Y, LIU B X, ZHANG D W , et al. Correlation,seasonal and temporal variation of water-soluble ions of PM2.5 in Beijing during 2012-2013[J]. Environmental Science, 2015,36(3):768-773. [13] 刘保献, 杨懂艳, 张大伟 , 等. 北京城区大气PM2.5主要化学组分构成研究[J]. 环境科学, 2015,36(7):2346-2351.LIU B X, YANG D Y, ZHANG D W , et al. Chemical species of PM2.5 in the urban area of Beijing[J]. Environmental Science, 2015,36(7):2346-2351. [14] 邓利群, 李红, 柴发合 , 等. 北京东北部城区大气细粒子与相关气体污染特征研究[J]. 中国环境科学, 2011,31(7):1064-1070.DENG L Q, LI H, CHAI F H , et al. The pollution characteristics of the atmospheric fime particles and related gaseous pollutants in the northeastern urban area of Beijing[J]. China Environmental Science, 2011,31(7):1064-1070. [15] KANG C H, KIM W H, KO H J , et al. Asian dust effects on total suspended particulate(TSP) compositions at Gosan in Jeju Island,Korea[J]. Atmospheric Research, 2009,94(2):345-355. [16] ZHANG D, IWASAKA Y . Nitrate and sulfate in individual Asian duststorm particles in Beijing,China in spring of 1995 and 1996[J]. Atmospheric Environment, 1999,33(19):3213-3223. [17] 乔佳佳, 祁建华, 刘苗苗 , 等. 青岛采暖期不同天气状况下大气颗粒态无机氮分布研究[J]. 环境科学, 2010,31(1):29-35.QIAO J J, QI J H, LIU M M , et al. Distribution of atmospheric particulate inorganic nitrogen in different weather conditions in the heating period in Qingdao[J]. Environmental Science, 2010,31(1):29-35. [18] 孙峰, 张大伟, 孙瑞雯 , 等. 北京地区冬季典型PM2.5重污染案例分析[J]. 中国环境监测, 2014,30(6):1-12.SUN F, ZHANG D W, SUN R W , et al. Typical heavy pollution episode analysis on PM2.5 in winter of Beijing[J]. Environmental Monitoring in China, 2014,30(6):1-12. [19] DLUGI R, JORDAN S, LINDEMANN E . The heterogeneous formation of sulfate aerosols in the atmosphere[J]. Journal of Aerosol Science, 1981,12(3):185-197. [20] 杨素霞, 曹军骥, 沈振兴 , 等. 西安冬、夏季PM2.5中水溶性无机离子的变化特征[J]. 环境化学, 2012,31(8):1179-1188.YANG S X, CAO J J, SHEN Z X , et al. Variations of water-soluble ions in PM2.5 at Xi'an between summer and winter[J]. Environmental Chemistry, 2012,31(8):1179-1188. [21] 李令军, 王英, 李金香 , 等. 2000—2010北京大气重污染研究[J]. 中国环境科学, 2012,32(1):23-30.LI L J, WANG Y, LI J X , et al. The analysis of heavy air pollution in Beijing during 2000-2010[J]. China Environmental Science, 2012,32(1):23-30. [22] 韩月梅, 沈振兴, 曹军骥 , 等. 西安市大气颗粒物中水溶性无机离子的季节变化特征[J]. 环境化学, 2009,28(2):261-266.HAN Y M, SHEN Z X, CAO J J , et al. Seasonal variations of water-soluble inorganic ions in atmospheric particles over Xi'an[J]. Environmental Chemistry, 2009,28(2):261-266. [23] WANG Y, ZHUANG G, SUN Y , et al. Water-soluble part of the aerosol in the dustorm season-evidence of the mixing between mineral and pollution aerosols[J]. Atmospheric Environment, 2005,39(37):7020-7029 [24] 北京市生态环境局. 2018年北京市生态环境状况公报[A∕OL].(2018-05-09)[2019-04-13]. [25] WANG Y, ZHUANG G S, ZHANG X Y , et al. The ion chemistry,seasonal cycle,and sources of PM2.5 and TSP aerosol in Shanghai[J]. Atmospheric Environment, 2006,40(16):2935-2952. [26] TRUEX T J, PIERSON W R, MCKEE D E . Sulfate in dieselexhaust[J]. Environment Science & Technology, 1980,14(9):1118-1121. [27] OHTA S, OKITA T A . Cheical characterization of atmospheric aerosol in Sapporo[J]. Atmospheric Environment Part A:General Topics, 1990,24(4):815-822. [28] 李伟芳, 白志鹏, 魏静东 , 等. 天津冬季大气中PM2.5及其主要组分的污染特征[J]. 中国环境科学, 2008,28(6):481-486.LI W F, BAI Z P, WEI J D , et al. Pollution characteristics of PM2.5 and its main components in Tianjin winter atmosphere[J]. China Environmental Science, 2008,28(6):481-486. [29] 王占山, 刘保献, 魏强 , 等. 北京市PM2.5二次水溶性无机离子变化特征[J]. 环境工程, 2016,34(4):105-109.WANG Z S, LIU B X, WEI Q , et al. Variation characteristics of secondary water-soluble inorganic ions in PM2.5 in Beijing[J]. Environmental Engineering, 2016,34(4):105-109. [30] 李丽珍, 沈振兴, 杜娜 , 等. 霾和正常天气下西安大气颗粒物中水溶性离子特征[J]. 中国科学院研究生院学报, 2007,24(5):674-679.LI L Z, SHEN Z X, DU N , et al. Chemical composition of water-soluble species between haze and normal days over Xi'an[J]. Journal of the Graduate School of the Chinese Academy of Sciences, 2007,24(5):674-679. [31] ZHANG W, CAPPS S L, HU Y , et al. Development of the high-orderdecoupled direct method in three dimensions for particulate matter:enabling advanced sensitivity analysis in air quality models[J]. Geoscientific Model Development, 2012,5(2):355-368. [32] 秦伟良, 许影 . 基于地统计学的江苏PM2.5空间变异性分析[J]. 环境工程, 2014,32(1):73-76.QIN W L, XU Y . Spatial variation of PM2.5 in Jiangsu Province based on geostatistical analysis[J]. Environmental Engineering, 2014,32(1):73-76. [33] 梁增强, 马民涛, 杜改芳 . 2003—2012年京津石三市大气污染特征及趋势对比[J]. 环境工程, 2014,32(12):76-81.LIANG Z Q, MA M T, DU G F . Comparison of characteristics and trend analysis of atompheric pollution in Beijing-Tianjin-Shijiazhuang,during 2003-2012[J]. Environmental Engineering, 2014,32(12):76-81. [34] 孙韧, 张文具, 董海燕 , 等. 天津市PM10和P M 2 . 5 中水溶性无机离子化学特征及来源分析 [J]. 中国环境监测, 2014,30(2):145-150.SUN R, ZHANG W J, DONG H Y , et al. Chemical character and source analysis of water-soluble irons in PM10 and PM2.5 in Tianjin City[J]. Environmental Monitoring in China, 2014,30(2):145-150. [35] 沈振兴, 韩月梅, 周娟 , 等. 西安冬季大气亚微米颗粒物的化学特征及来源解析[J]. 西安交通大学学报, 2008,42(11):1418-1423.SHEN Z X, HAN Y M, ZHOU J , et al. Chemical composition and source identification of submicron particles over Xi'an during winter[J]. Journal of Xi'an Jiaotong University, 2008,42(11):1418-1423. [36] 李英红, 谭吉华, 饶志国 , 等. 兰州市大气细颗粒物中水溶性离子的污染特征[J]. 环境化学, 2016,35(9):1799-1807.LI Y H, TAN J H, RAO Z G , et al. Pollution characteristics of water soluble ions in atmospheric fine particles in Lanzhou[J]. Environmental Chemistry, 2016,35(9):1799-1807. [37] 李伟芳 . 天津PM2.5理化特性和含碳气溶胶的分布与来源研究[D]. 天津:南开大学, 2008. [38] 安欣欣, 张大伟, 冯鹏 , 等. 北京城区夏季PM2.5中碳组分和二次水溶性无机离子浓度特征[J]. 环境化学, 2016,35(4):713-720.AN X X, ZHANG D W, FENG P , et al. Characteristics of carbon components and secondary water-soluble inorganic ions in PM2.5 in summer in urban Beijing[J]. Environmental Chemistry, 2016,35(4):713-720. [39] SEINFELD J H, PANDIS S N . Atmospheric chemistry and physics:from air pollution to climate change[M]. New York:John Wiley & Sons, 1996: 379-383. [40] 孟琛琛, 王丽涛, 张芬芬 , 等. 邯郸市PM2.5中水溶性无机离子污染特征及来源解析[J]. 环境科学学报, 2015,35(11):3443-3451.MENG C C, WANG L T, ZHANG F F , et al. Pollution characteristics and source apportionment of water soluble inorganic ions in PM2.5 in Handan City[J]. Acta Scientiae Circumstantiae, 2015,35(11):3443-3451. [41] 栾玉荣 . 我国多站点主要水溶性气溶胶的空间分布和时间变化特征[D]. 北京:中国气象科学研究, 2008.
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