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油基钻井岩屑固化体中多环芳烃释放特征

王之超 何洁 张曼丽 蔡洪英 黄泽春

王之超, 何洁, 张曼丽, 蔡洪英, 黄泽春. 油基钻井岩屑固化体中多环芳烃释放特征[J]. 环境工程技术学报, 2020, 10(4): 647-652. doi: 10.12153/j.issn.1674-991X.20200013
引用本文: 王之超, 何洁, 张曼丽, 蔡洪英, 黄泽春. 油基钻井岩屑固化体中多环芳烃释放特征[J]. 环境工程技术学报, 2020, 10(4): 647-652. doi: 10.12153/j.issn.1674-991X.20200013
WANG Zhichao, HE Jie, ZHANG Manli, CAI Hongying, HUANG Zechun. Release characteristics of PAHs in oil-based drilling cuttings solidified body[J]. Journal of Environmental Engineering Technology, 2020, 10(4): 647-652. doi: 10.12153/j.issn.1674-991X.20200013
Citation: WANG Zhichao, HE Jie, ZHANG Manli, CAI Hongying, HUANG Zechun. Release characteristics of PAHs in oil-based drilling cuttings solidified body[J]. Journal of Environmental Engineering Technology, 2020, 10(4): 647-652. doi: 10.12153/j.issn.1674-991X.20200013

油基钻井岩屑固化体中多环芳烃释放特征

doi: 10.12153/j.issn.1674-991X.20200013
详细信息
    作者简介:

    王之超(1994—),男,硕士研究生,主要研究方向为固体废物处置及资源化利用,1973753012@qq.com

    通讯作者:

    黄泽春 E-mail: huangzc@craes.org.cn

  • 中图分类号: X705

Release characteristics of PAHs in oil-based drilling cuttings solidified body

More Information
    Corresponding author: HUANG Zechun E-mail: huangzc@craes.org.cn
  • 摘要: 油基钻井岩屑资源化利用的有效方式是制备成块状固化体,但固化体在应用过程中存在多环芳烃浸出的风险。采用固体中无机组分有效量测试(NEN7371)方法和块状材料中无机组分的扩散实验(NEN7375)方法,研究固化体内萘、蒽、荧蒽、苯并(b)荧蒽和苯并(a)芘5种多环芳烃的释放特性,评估其浸出释放风险。结果表明:5种多环芳烃的有效释放率均在2%以下,其中苯并(a)芘有效释放率最高,浸出液中浓度超过GB/T 14848—2017《地下水质量标准》中Ⅲ类限值;在静态浸泡释放特征试验中,5种多环芳烃的释放集中在浸出前期,前16 d累积释放量占64 d累积释放总量的比值均超过78%;5种多环芳烃释放机理包括扩散控制、溶解释放、延滞释放、耗竭和表面冲刷,固化体中不同多环芳烃释放特征存在一定的差异,但总体上以扩散控制为主,后期均表现为耗竭机制。

     

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出版历程
  • 收稿日期:  2020-02-09
  • 刊出日期:  2020-07-20

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