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黄淮平原典型城市农业氨排放清单及特征分析——以亳州市为例

陈雯 薛志钢 营娜 张皓 续鹏 杨丽 杜谨宏 石应杰

陈雯, 薛志钢, 营娜, 张皓, 续鹏, 杨丽, 杜谨宏, 石应杰. 黄淮平原典型城市农业氨排放清单及特征分析——以亳州市为例[J]. 环境工程技术学报, 2021, 11(3): 476-483. doi: 10.12153/j.issn.1674-991X.20210049
引用本文: 陈雯, 薛志钢, 营娜, 张皓, 续鹏, 杨丽, 杜谨宏, 石应杰. 黄淮平原典型城市农业氨排放清单及特征分析——以亳州市为例[J]. 环境工程技术学报, 2021, 11(3): 476-483. doi: 10.12153/j.issn.1674-991X.20210049
CHEN Wen, XUE Zhigang, YING Na, ZHANG Hao, XU Peng, YANG Li, DU Jinhong, SHI Yingjie. Agricultural ammonia emission inventory and characteristics analysis of typical cities in Huanghuai Plain: take Bozhou City as an example[J]. Journal of Environmental Engineering Technology, 2021, 11(3): 476-483. doi: 10.12153/j.issn.1674-991X.20210049
Citation: CHEN Wen, XUE Zhigang, YING Na, ZHANG Hao, XU Peng, YANG Li, DU Jinhong, SHI Yingjie. Agricultural ammonia emission inventory and characteristics analysis of typical cities in Huanghuai Plain: take Bozhou City as an example[J]. Journal of Environmental Engineering Technology, 2021, 11(3): 476-483. doi: 10.12153/j.issn.1674-991X.20210049

黄淮平原典型城市农业氨排放清单及特征分析——以亳州市为例

doi: 10.12153/j.issn.1674-991X.20210049
详细信息
    作者简介:

    陈雯(1995—),女,硕士研究生,主要研究方向为大气污染源清单编制及校核,1929579589@qq.com

    通讯作者:

    薛志钢 E-mail: xuezg@craes.org.cn

Agricultural ammonia emission inventory and characteristics analysis of typical cities in Huanghuai Plain: take Bozhou City as an example

More Information
    Corresponding author: XUE Zhigang E-mail: xuezg@craes.org.cn
  • 摘要: 亳州市是黄淮平原典型城市,而农业是其最大的氨排放来源。基于亳州市畜禽养殖、氮肥施用、固氮植物、土壤本底、秸秆堆肥、人体粪便6类农业源活动水平数据与排放因子,建立2011—2018年亳州市农业源氨排放清单,分析该市氨排放结构、空间分布、历年变化趋势及不确定性,进一步深入了解黄淮平原典型城市农业氨排放特征。结果表明:2018年亳州市农业氨排放总量为27 529.19 t/a,其中畜禽养殖与氮肥施用是农业氨排放量较大的2类源,占比分别为68.81%、16.85%。农业氨排放集中在利辛县与谯城区,分别占全市总排放量的28.9%、27.8%。亳州市农业氨排放量从2011年的35 097.97 t/a小幅升至2014年的38 441.13 t/a,2015—2017年变化不大,2018年降至27 529.19 t/a。从各类农业源氨排放量变化趋势来看,2011—2018年秸秆堆肥、土壤本底的氨排放量出现微小涨幅,畜禽养殖、氮肥施用、固氮植物、人体粪便的氨排放量呈下降趋势。此外,2011—2018年亳州市农业源清单的不确定性处于-22%~26%,清单不确定性较小。

     

  • [1] HAMAOUI-LAGUEL L, MELEUX F, BEEKMANN M, et al. Improving ammonia emissions in air quality modelling for France[J]. Atmospheric Environment, 2014, 92:584-595.
    doi: 10.1016/j.atmosenv.2012.08.002
    [2] BISWAS K F, GHAURI B M, HUSAIN L. Gaseous and aerosol pollutants during fog and clear episodes in South Asian urban atmosphere[J]. Atmospheric Environment, 2008, 42(33):7775-7785.
    doi: 10.1016/j.atmosenv.2008.04.056
    [3] FANG M, CHAN C K, YAO X H. Managing air quality in a rapidly developing nation:China[J]. Atmospheric Environment, 2009, 43(1):79-86.
    doi: 10.1016/j.atmosenv.2008.09.064
    [4] BATTYE W, ANEJA V P, ROELLE P A. Evaluation and improvement of ammonia emissions inventories[J]. Atmospheric Environment, 2003, 37(27):3873-3883.
    doi: 10.1016/S1352-2310(03)00343-1
    [5] PUI D Y H, CHEN S C, ZUO Z L. PM2.5 in China:measurements,sources,visibility and health effects,and mitigation [J]. Particuology, 2014, 13:1-26.
    doi: 10.1016/j.partic.2013.11.001
    [6] YE X N, MA Z, ZHANG J C, et al. Important role of ammonia on haze formation in Shanghai[J]. Environmental Research Letters, 2011, 6(2):024019.
    doi: 10.1088/1748-9326/6/2/024019
    [7] CHARLSON R J, SCHWARTZ S E, HALES J M, et al. Climate forcing by anthropogenic aerosols[J]. Science, 1992, 255:423-430.
    doi: 10.1126/science.255.5043.423
    [8] KIRKBY J, CURTIUS J, ALMEIDA J, et al. Role of sulphuric acid,ammonia and galactic cosmic rays in atmospheric aerosol nucleation[J]. Nature, 2011, 476:429-433.
    doi: 10.1038/nature10343
    [9] KULMALA M. Aerosol formation during PARFORCE:ternary nucleation of H2SO4,NH3,and H2O [J]. Journal of Geophysical Research Atmospheres, 2002, 107(19):8111.
    doi: 10.1029/2001JD000900
    [10] ANEJA V P, NELSON D R, ROELLE P A, et al. Agricultural ammonia emissions and ammonium concentrations associated with aerosols and precipitation in the Southeast United States[J]. Journal of Geophysical Research Atmospheres, 2003.doi: 10.1029/2002JD002271.
    doi: 10.1029/2002JD002271
    [11] BEHERA S N, SHARMA M, ANEJA V P, et al. Ammonia in the atmosphere:a review on emission sources,atmospheric chemistry and deposition on terrestrial bodies[J]. Environmental Science and Pollution Research, 2013, 20(11):8092-8131.
    doi: 10.1007/s11356-013-2051-9
    [12] HELLSTEN S, DRAGOSITS U, PLACE C J, et al. Modelling the spatial distribution of ammonia emissions in the UK[J]. Environmental Pollution, 2008, 154(3):370-379.
    doi: 10.1016/j.envpol.2008.02.017
    [13] ZHAO D W, WANG A P. Estimation of anthropogenic ammonia emissions in Asia[J]. Atmospheric Environment, 1994, 28(4):689-694.
    doi: 10.1016/1352-2310(94)90045-0
    [14] HUANG X, SONG Y, LI M M, et al. A high-resolution ammonia emission inventory in China[J]. Global Biogeochemical Cycles, 2012.doi: 10.1029/2011gb004161.
    [15] ZHANG L, CHEN Y F, ZHAO Y H, et al. Agricultural ammonia emissions in China:reconciling bottom-up and top-downestimates[J]. Atmospheric Chemistry and Physics, 2018, 18(1):339-355.
    doi: 10.5194/acp-18-339-2018
    [16] MA S Y. High-resolution assessment of ammonia emissions in China:inventories,driving forces and mitigation[J]. Atmospheric Environment, 2020, 229:117458.
    doi: 10.1016/j.atmosenv.2020.117458
    [17] XU P, ZHANG Y S, GONG W W, et al. An inventory of the emission of ammonia from agricultural fertilizer application in China for 2010 and its high-resolution spatial distribution[J]. Atmospheric Environment,2015, 115:141-148.
    doi: 10.1016/j.atmosenv.2015.05.020
    [18] 董艳强, 陈长虹, 黄成, 等. 长江三角洲地区人为源氨排放清单及分布特征[J]. 环境科学学报, 2009, 29(8):1611-1617.

    DONG Y Q, CHEN C H, HUANG C, et al. Anthropogenic emissions and distribution of ammonia over the Yangtze River Delta[J]. Acta Scientiae Circumstantiae, 2009, 29(8):1611-1617.
    [19] 尹沙沙, 郑君瑜, 张礼俊, 等. 珠江三角洲人为氨源排放清单及特征[J]. 环境科学, 2010, 31(5):1146-1151.

    YIN S S, ZHENG J Y, ZHANG L J, et al. Anthropogenic ammonia emission inventory and characteristics in the Pearl River Delta Region[J]. Environmental Science, 2010, 31(5):1146-1151.
    [20] ZHOU Y, CHENG S Y, LANG J L, et al. A comprehensive ammonia emission inventory with high-resolution and its evaluation in the Beijing-Tianjin-Hebei(BTH)Region,China[J]. Atmospheric Environment, 2015, 106:305-317.
    doi: 10.1016/j.atmosenv.2015.01.069
    [21] 覃思, 孔少飞, 吴剑, 等. 1996—2016年湖北省氨排放时空差异及影响因素[J]. 中国环境科学, 2020, 40(4):1403-1413.

    QIN S, KONG S F, WU J, et al. Spatial-temporal diversities of ammonia emissions and impacting factors in Hubei Province from 1996 to 2016[J]. China Environmental Science,2020, 40(4):1403-1413.
    [22] 侯新红, 于兴娜, 沈丽, 等. 2013—2017年江苏省人为源氨排放清单的建立及特征[J]. 环境科学, 2019, 40(11):4862-4869.

    HOU X H, YU X N, SHEN L, et al. Establishment and characteristics of an artificial ammonia emissions inventory in Jiangsu Province from 2013 to 2017[J]. Environmental Science,2019, 40(11):4862-4869.
    [23] WANG C, YIN S S, BAI L, et al. High-resolution ammonia emission inventories with comprehensive analysis and evaluation in Henan,China, 2006-2016[J]. Atmospheric Environment,2018, 193:11-23.
    doi: 10.1016/j.atmosenv.2018.08.063
    [24] 刘春蕾, 杨峰. 南京市2013年人为源大气氨排放清单及特征[J]. 安徽农业科学, 2015, 43(29):263-266.

    LIU C L, YANG F. Nanjing anthropogenic ammonia emission inventory and its characteristics in 2013[J]. Journal of Anhui Agricultural Sciences, 2015, 43(29):263-266.
    [25] 周静, 刘松华, 谭译, 等. 苏州市人为源氨排放清单及其分布特征[J]. 环境科学研究, 2016, 29(8):1137-1144.

    ZHOU J, LIU S H, TAN Y, et al. Anthropogenic ammonia emission inventory and its spatial distribution in Suzhou City[J]. Research of Environmental Sciences, 2016, 29(8):1137-1144.
    [26] 苏航, 闫东杰, 黄学敏, 等. 西安市人为源大气氨排放清单及特征[J]. 环境科学, 2016, 37(11):4117-4123.

    SU H, YAN D J, HUANG X M, et al. Inventory and characteristics of anthropogenic ammonia emission in Xi’an[J]. Environmental Science, 2016, 37(11):4117-4123.
    [27] 董婧, 孙长虹, 王永刚, 等. 北京市典型农业区域大气环境氨浓度动态变化分析[J]. 环境工程技术学报, 2017, 7(3):262-267.

    DONG J, SUN C H, WANG Y G, et al. Dynamics of atmospheric ammonia concentrations over representative agricultural region in Beijing[J]. Journal of Environmental Engineering Technology, 2017, 7(3):262-267.
    [28] 生态环境部. 大气氨源排放清单编制技术指南(试行)[A/OL].(2014-08-20)[2020-08-10]. http://www.mee.gov.cn/gkml/hbb/bgg/201408/W020140828351293771578.pdf.
    [29] JU X T, XING G X, CHEN X P, et al. Reducing environmental risk by improving N management in intensive Chinese agricultural systems[J]. PNAS, 2009, 106(19):8077.
    doi: 10.1073/pnas.0902655106
    [30] 高榕. 山东省农业源氨排放清单及其减排潜力研究[D]. 济南: 济南大学, 2018:15-58.
    [31] KANG Y N, LIU M X, SONG Y, et al. High-resolution ammonia emissions inventories in China from 1980 to 2012[J]. Atmospheric Chemistry and Physics,2016, 16(4):2043-2058.
    doi: 10.5194/acp-16-2043-2016
    [32] 尤翔宇, 刘湛, 张青梅, 等. 长株潭地区人为源氨排放清单及分布特征[J]. 环境科学, 2016, 37(1):94-101.

    YOU X Y, LIU Z, ZHANG Q M, et al. Anthropogenic ammonia emission inventory and its spatial distribution in Chang-Zhu-Tan Region[J]. Environmental Science, 2016, 37(1):94-101.
    [33] 郑志侠, 翁建宇, 汪水兵, 等. 安徽省农田生态系统氨排放研究[J]. 安徽农业大学学报, 2016, 43(4):562-567.

    ZHENG Z X, WENG J Y, WANG S B, et al. Study on ammonia emission from the farmland ecosystem in Anhui Province[J]. Journal of Anhui Agricultural University, 2016, 43(4):562-567.
    [34] 周伟. 前三季度全省农业生产总体平稳生猪产能大幅下滑[EB/OL].( 2019-11-12)[ 2021-02-08]. http://tjj.ah.gov.cn/public/6981/145100191.html.
    [35] 陈丹丹. 亳州市大多数规模养殖场已完成整改任务[EB/OL].( 2018-08-31)[ 2021-02-08]. http://ah.ifeng.com/a/20180831/6847812_0.shtml.
    [36] 管梦爽. 忻州市人为源VOC S物种排放清单及不确定性分析 [D]. 北京: 华北电力大学(北京), 2019:4-5.
    [37] HOU X H, YU X N. An ammonia emissions inventory for agricultural sources in Hefei,China[J]. Atmospheric and Oceanic Science Letters, 2020, 13(3):260-267.
    doi: 10.1080/16742834.2020.1747355
    [38] MISSELBROOK T H, SUTTON M A, SCHOLEFIELD D. A simple process-based model for estimating ammonia emissions from agricultural land after fertilizer applications[J]. Soil Use and Management, 2006, 20(4):365-372.
    doi: 10.1111/j.1475-2743.2004.tb00385.x
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  • 收稿日期:  2021-02-26
  • 刊出日期:  2021-05-20

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