Investigation on air pollutants and carbon dioxide emissions from motor vehicles in Beijing based on COPERT model
-
摘要: 机动车大气污染物及CO2减排对于改善空气质量和缓解气候变化具有重要的作用。综合利用北京市机动车保有量、道路行驶工况、气象、燃料组分及燃料消耗量等数据,应用COPERT模型计算得到北京市机动车主要大气污染物和CO2排放量,并识别其污染排放特征和不同车型、排放标准等级车辆的排放贡献,采用ADMS-Urban模型模拟了机动车污染排放对周边环境的影响。结果表明:2019年北京市机动车4项主要大气污染物CO、NOx、PM2.5和VOCs排放量分别为12.15万、4.06万、0.18万和2.57万t。车辆结构得到优化,国四及以上排放标准车辆占比达86.97%,数量占4%的柴油客货车排放贡献大,分别占机动车NOx和PM2.5排放总量的84%和60%;非末端排放占机动车VOCs排放量的20%,需要引起关注。机动车尾气排放对5个交通监测站点贡献的NO2平均浓度为15.7 μg/m3,其对环境质量影响较大;机动车CO2排放量为1 683万t,其中柴油车排放贡献约21%。对北京市机动车大气污染物和碳排放需要进一步协同控制。Abstract: Air pollutants and carbon dioxide (CO2) emissions reduction from motor vehicles play an important role in improving air quality and mitigating climate change. The data of vehicle population, road-driving conditions, meteorological, fuel composition and fuel consumption were comprehensively used to calculate the main air pollutants and CO2 emissions of motor vehicles in Beijing based on COPERT Model. The emission characteristics, emission contribution of the vehicles of different types, and emission standard levels were identified. Urban-ADMS model was used to simulate and quantify the effect on surrounding environment by motor vehicles. The results showed that: the emissions of CO, NOx, PM2.5 and VOCs from motor vehicles of Beijing was 121 500, 40 600, 1 800 and 25 700 tons, respectively, in 2019. The structure of vehicles had been optimized. Vehicles with National IV and above standards accounted for 86.97%. Diesel passenger and freight vehicles accounting for 4% contributed greatly to the emissions, accounting for 84% and 60% of the total emissions of NOx and PM2.5, respectively. Evaporative emissions from gasoline vehicles accounted for 20% of VOCs emissions from motor vehicles, which required attention. Vehicle exhaust emissions contributed 15.7 μg/m3 to the average NO2 concentration at five traffic monitoring stations which had a great impact on air quality. CO2 emissions of motor vehicles were 16.83 million tons, of which diesel vehicle emissions contributed about 21%. Air pollutants and carbon emissions of motor vehicles need further coordinated control.
-
Key words:
- COPERT model /
- Beijing /
- motor vehicle /
- air pollution /
- carbon dioxide
-
[1] CAI H, XIE S D. Estimation of vehicular emission inventories in China from 1980 to 2005[J]. Atmospheric Environment, 2007, 41(39):8963-8979.
doi: 10.1016/j.atmosenv.2007.08.019[2] RICHTER A, BURROWS J P, NÜSS H, et al. Increase in tropospheric nitrogen dioxide over China observed from space[J]. Nature, 2005, 437:129-132.
doi: 10.1038/nature04092[3] BROWN S G, FRANKEL A, HAFNER H R. Source apportionment of VOCs in the Los Angeles area using positive matrix factorization[J]. Atmospheric Environment, 2007, 41(2):227-237.
doi: 10.1016/j.atmosenv.2006.08.021[4] 解淑霞, 黄志辉, 王鑫, 等. 阳泉市2017年基于交通流量的机动车排放清单[J]. 环境工程技术学报, 2021, 11(2):226-233.XIE S X, HUANG Z H, WANG X, et al. Emission inventory of motor vehicle based on traffic flow for Yangquan City in 2017[J]. Journal of Environmental Engineering Technology, 2021, 11(2):226-233. [5] LADEN F, NEAS L M, DOCKERY D W, et al. Association of fine particulate matter from different sources with daily mortality in six US cities[J]. Environmental Health Perspectives, 2000, 108(10):941-947.
doi: 10.1289/ehp.00108941[6] 王燕军, 何巍楠, 宋国华, 等. 北京市2017年典型日机动车动态排放特征研究[J]. 环境科学研究, 2021, 34(1):141-148.WANG Y J, HE W N, SONG G H, et al. Vehicular dynamic emission characteristics of typical days in Beijing in 2017[J]. Research of Environmental Sciences, 2021, 34(1):141-148. [7] 王凯, 樊守彬, 孙改红, 等. 基于行驶里程的北京市延庆区机动车排放清单建立及特征分析[J]. 环境工程技术学报, 2019, 9(2):119-125.WANG K, FAN S B, SUN G H, et al. Motor vehicles emission inventory at county level based on vehicle kilometers travel:a case study of Yanqing District of Beijing[J]. Journal of Environmental Engineering Technology, 2019, 9(2):119-125. [8] 樊守彬, 田灵娣, 张东旭. 基于COPERT模式的北京市汽油车蒸发VOCs排放清单[J]. 环境工程学报, 2016, 10(6):3091-3096.FAN S B, TIAN L D, ZHANG D X. Emission inventory of gasoline evaporation from vehicles in Beijing based on COPERT model[J]. Chinese Journal of Environmental Engineering, 2016, 10(6):3091-3096. [9] HE L, ZHU J, QIAN Y, et al. Study on pollutants emission characteristics of vehicles in Urumqi[J]. Environmental Engineering, 2015, 33(5):90-94. [10] 王孝文, 田伟利, 张清宇. 杭州市机动车污染物排放清单的建立[J]. 中国环境科学, 2012, 32(8):1368-1374.WANG X W, TIAN W L, ZHANG Q Y. Development of motor vehicles emission inventory in Hangzhou[J]. China Environmental Science, 2012, 32(8):1368-1374. [11] YANG W, YU C Y, YUAN W, et al. High-resolution vehicle emission inventory and emission control policy scenario analysis,a case in the Beijing-Tianjin-Hebei (BTH) Region,China[J]. Journal of Cleaner Production, 2018, 203:530-539.
doi: 10.1016/j.jclepro.2018.08.256[12] DEY S, CAULFIELD B, GHOSH B. Modelling uncertainty of vehicular emissions inventory:a case study of Ireland[J]. Journal of Cleaner Production, 2019, 213:1115-1126.
doi: 10.1016/j.jclepro.2018.12.125[13] ZHANG S J, WU Y, HUANG R K, et al. High-resolution simulation of link-level vehicle emissions and concentrations for air pollutants in a traffic-populated eastern Asian city[J]. Atmospheric Chemistry and Physics, 2016, 16(15):9965-9981. [14] 纪亮, 袁盈, 李刚, 等. 我国机动车排放标准的大气污染物减排效果研究[J]. 环境工程技术学报, 2011, 1(3):237-242.JI L A, YUAN Y, LI G, et al. Study on emission reduction effect of motor vehicle emission standards in China[J]. Journal of Environmental Engineering Technology, 2011, 1(3):237-242. [15] 蔡皓, 谢绍东. 中国不同排放标准机动车排放因子的确定[J]. 北京大学学报(自然科学版), 2010, 46(3):319-326.CAI H, XIE S D. Determination of emission factors from motor vehicles under different emission standards in China[J]. Acta Scientiarum Naturalium Universitatis Pekinensis, 2010, 46(3):319-326. [16] 谢绍东, 宋翔宇, 申新华. 应用COPERTⅢ模型计算中国机动车排放因子[J]. 环境科学, 2006, 27(3):415-419.XIE S D, SONG X Y, SHEN X H. Calculating vehicular emission factors with COPERTⅢ mode in China[J]. Environmental Science, 2006, 27(3):415-419. [17] 王聪. 基于COPERT4模型的山东省汽车尾气排放特征及预测研究[D]. 青岛:中国海洋大学, 2015. [18] KOUSOULIDOU M, NTZIACHRISTOS L, MELLIOS G, et al. Road-transport emission projections to 2020 in European urban environments[J]. Atmospheric Environment, 2008, 42(32):7465-7475.
doi: 10.1016/j.atmosenv.2008.06.002[19] 樊守彬. 北京机动车尾气排放特征研究[J]. 环境科学与管理, 2011, 36(4):28-31.FAN S B. Tail-pipe emission characteristics from on-road vehicles in Beijing[J]. Environmental Science and Management, 2011, 36(4):28-31. [20] 徐伟嘉, 黄建彰, 刘永红, 等. 基于PEMS与COPERT的机动车尾气排放特征分析[J]. 环境科学与技术, 2014, 37(增刊 1):77-81.XU W J, HUANG J Z, LIU Y H, et al. Study on the characteristics of traffic emission with PEMS and COPERT[J]. Environmental Science & Technology, 2014, 37(Suppl 1):77-81. [21] TANG G Q, CHAO N, WANG Y S, et al. Vehicular emissions in China in 2006 and 2010[J]. Journal of Environmental Sciences, 2016, 48:179-192.
doi: 10.1016/j.jes.2016.01.031[22] 姚欣灿, 黄如娜, 农加进, 等. 广州市2010年道路机动车排放清单研究[J]. 广州环境科学, 2012(2):20-24.YAO X C, HUANG R N, NONG J J, et al. Vehicle emission inventory of Guangzhou in 2010[J]. Guangzhou Environmental Sciences, 2012(2):20-24. [23] 郝艳召, 邓顺熙, 邱兆文, 等. 基于MOVES模型的西安市机动车排放清单研究[J]. 环境污染与防治, 2017, 39(3):227-231.HAO Y Z, DENG S X, QIU Z W, et al. Vehicle emission inventory for Xi’an based on MOVES model[J]. Environmental Pollution & Control, 2017, 39(3):227-231. [24] 环境保护部. 道路机动车大气污染物排放清单编制技术指南(试行)[S/OL].[2021-04-20].http://www.mee.gov.cn/gkml/hbb/bgth/201407/W020140708387895271474.pdf . [25] 北京市统计局. 北京统计年鉴[A/OL].[2021-04-20].http://nj.tjj.beijing.gov.cn/nj/main/2019-tjnj/zk/indexch.htm , 2019-11-05. [26] 郭继孚. 2020北京市交通发展年度报告[R]. 北京:北京交通发展研究院, 2020. [27] 贺克斌. 城市大气污染物排放清单编制技术手册[EB/OL].[2021-04-20].https://max.book118.com/html/2018/1116/8107025055001133.shtm . 2015-4. [28] 茹宝琳. ADMS模型在大气环境影响评价中的应用[J]. 山东化工, 2018, 47(20):204-205.RU B L. Application of ADMS model in atmospheric environmental impact assessment[J]. Shandong Chemical Industry, 2018, 47(20):204-205. [29] 陶双成. 关中城市群道路移动源污染物排放清单与减排策略研究[D]. 西安:长安大学, 2016. [30] YAO Z, WEI H, PERUGU H, et al. Sensitivity analysis of project level MOVES running emission rates for light and heavy duty vehicles[J]. Journal of Traffic and Transportation Engineering (English Edition), 2014, 1(2):81-96. [31] ESTEVES-BOOTH A, MUNEER T, KUBIE J, et al. A review of vehicular emission models and driving cycles[J]. Proceedings of the Institution of Mechanical Engineers,Part C:Journal of Mechanical Engineering Science, 2002, 216(8):777-797.
doi: 10.1243/09544060260171429[32] LANG J L, CHENG S Y, ZHOU Y, et al. Air pollutant emissions from on-road vehicles in China,1999-2011[J]. Science of the Total Environment, 2014, 496:1-10.
doi: 10.1016/j.scitotenv.2014.07.021[33] ZHENG J Y, ZHANG L J, CHE W W, et al. A highly resolved temporal and spatial air pollutant emission inventory for the Pearl River Delta region,China and its uncertainty assessment[J]. Atmospheric Environment, 2009, 43(32):5112-5122.
doi: 10.1016/j.atmosenv.2009.04.060[34] WANG H K, CHEN C H, HUANG C, et al. On-road vehicle emission inventory and its uncertainty analysis for Shanghai,China[J]. Science of the Total Environment, 2008, 398(1/2/3):60-67.
doi: 10.1016/j.scitotenv.2008.01.038
点击查看大图
计量
- 文章访问数: 1294
- HTML全文浏览量: 316
- PDF下载量: 173
- 被引次数: 0