移动监测技术在大气环境研究中的应用

朱明玉; 初红涛; 高元官; 李刚; 全权浩; 蔡爀基; 赵刚; 张浩; 杨小阳

doi:10.12153/j.issn.1674-991X.20230604

移动监测技术在大气环境研究中的应用

doi: 10.12153/j.issn.1674-991X.20230604

朱明玉^{1, 2,},
初红涛¹,
高元官^2, ,,
李刚²,
全权浩³,
蔡爀基³,
赵刚²,
张浩²,
杨小阳²

1.
齐齐哈尔大学化学与化学工程学院
2.
中国环境科学研究院大气环境研究所
3.
韩国国立环境科学院

基金项目: 国家重点研发计划项目（2023YFC3705804）；中韩合作“晴天计划”项目

详细信息

作者简介:
朱明玉（1998—），女，硕士研究生，主要从事大气环境的移动监测研究，935512230@qq.com

通讯作者:
高元官（1990—），男，工程师，主要从事城市大气环境污染治理相关研究，gaoyg@craes.org.cn

中图分类号: X831
计量
- 文章访问数: 121
- HTML全文浏览量: 41
- PDF下载量: 49
- 被引次数: 0
出版历程
- 收稿日期: 2023-08-18
- 录用日期: 2024-01-16
- 修回日期: 2023-10-18

Application of mobile monitoring technology in atmospheric environment research

1.
School of Chemistry and Chemistry Engineering, Qiqihar University
2.
Atmospheric Environment Institute, Chinese Research Academy of Environmental Sciences
3.
National Institute of Envrionmental Research (NIER)

摘要

摘要:
移动监测是把用于环境监测的设备安装在移动载体（汽车、自行车、无人机和船等）上，开展环境质量监测的技术。移动监测技术以其灵活、机动、及时等优势，近年来被广泛应用于大气环境监测中，但针对移动监测技术在大气环境研究中的应用场景及其存在的优缺点等缺少系统性研究。通过文献调研的方式对国内外移动监测技术在大气环境研究中的应用进行综述，重点讨论了监测设备及其搭载平台。将移动监测设备划分为传感器和大型设备2类，其中传感器以体积小、成本低等优势被大量应用在无人机、汽车等平台中。大型设备则包括监测仪和分析仪，但由于受到体积和成本的限制多被应用在飞机和船等面积较大的平台中。根据大气环境移动监测设备搭载的平台将其划分为车载移动监测、机载移动监测和船载移动监测三大类，其中车载移动监测主要用于环境质量监测、溯源分析和热点监测、汽车尾气排放监测及空气污染暴露监测等，机载移动监测主要用于环境空气质量监测、溯源分析和热点监测及大气污染物传输监测，船载移动监测主要用于海表大气组分、溯源分析和船舶尾气排放等研究。最后讨论了移动监测平台现有应用中存在的问题（例如覆盖率、续航、数据质量等），并对未来研究进行了展望。
- 气溶胶 /
- 空气质量监测 /
- 移动平台 /
- 传感器 /
- 研究进展
Abstract:
Mobile monitoring is a technique for conducting environmental quality assessments by deploying monitoring equipment on mobile platforms like cars, bicycles, unmanned aerial vehicles (UAVs) and boats. Due to its flexibility, mobility, and real-time capabilities, mobile monitoring technology has gained widespread application in recent years, particularly in atmospheric environmental monitoring. However, there is a shortage of systematic research regarding the application scenarios, advantages, and drawbacks of mobile monitoring technology in atmospheric environmental research. A literature-based review of the foreign and domestic applications of mobile monitoring technology in atmospheric environmental research was conducted, with a focus on the monitoring equipment and the platforms used for atmospheric environmental mobile monitoring. The mobile monitoring equipment is categorized into two groups: sensors and large-scale devices. Sensors, characterized by their compact size and cost-effectiveness, find extensive use on platforms like UAVs and automobiles. Conversely, large-scale devices, including monitors and analyzers, are primarily employed on larger platforms like aircraft and ships, mainly due to size and cost constraints. Atmospheric environmental mobile monitoring platforms are classified into three categories: vehicle-based, aircraft-based, and ship-based. Vehicle-based mobile monitoring is primarily employed for environmental quality assessment, traceability analysis, hotspot monitoring, vehicle emissions tracking, and air pollution exposure measurement. Aircraft platforms play a key role in monitoring ambient air quality, traceability analysis, hotspot monitoring, and the tracking of atmospheric pollutant dispersion. Ship-based mobile monitoring platforms are chiefly utilized for studying sea surface atmospheric components, traceability analysis, and ship exhaust emissions research. Finally, current challenges in existing applications of mobile monitoring platforms, such as coverage, battery life, and data quality, were addressed, and future perspectives were presented for the field.
- aerosols /
- air quality monitoring /
- mobile platform /
- sensors /
- research progress

HTML全文

表 1 移动监测平台的应用

Table 1. Application of mobile monitoring platforms

搭载平台	应用场景	内容
车载	环境空气质量监测	测量环境污染物浓度和绘制高分辨率污染地图
	溯源分析和热点监测	对污染峰值进行定位和对污染源进行分析
	汽车尾气排放监测	对汽车尾气排放进行在线监测
	空气污染暴露监测	在交通工具内对通勤过程中的污染物进行监测
机载	环境空气质量监测	对城市与自然环境空气的水平和垂直方向进行监测
	溯源分析和热点监测	对工业区、农业区等环境污染源进行定位分析
	大气污染物的传输监测	低层大气下污染物的水平和垂直传输监测
船载	海表大气组分监测	对海表大气的具体成分和浓度进行分析
	溯源分析	海洋气溶胶来源分析
	船舶排放监测	对船舶排放进行实船测试

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参考文献(97)

[1]	BOANINI C, MECCA D, POGNANT F, et al. Integrated mobile laboratory for air pollution assessment: literature review and cc-TrAIRer design[J]. Atmosphere,2021,12(8):1004. doi: 10.3390/atmos12081004
[2]	李冬, 陈建华, 张月帆, 等. 道路扬尘检测方法研究进展[J]. 环境工程技术学报,2021,11(3):537-545. LI D, CHEN J H, ZHANG Y F, et al. Research progress of detection methods of road dust[J]. Journal of Environmental Engineering Technology,2021,11(3):537-545.
[3]	KOLB C E, HERNDON S C, McMANUS J B, et al. Mobile laboratory with rapid response instruments for real-time measurements of urban and regional trace gas and particulate distributions and emission source characteristics[J]. Environmental Science & Technology,2004,38(21):5694-5703.
[4]	DIAS D, TCHEPEL O. Spatial and temporal dynamics in air pollution exposure assessment[J]. International Journal of Environmental Research and Public Health,2018,15(3):558. doi: 10.3390/ijerph15030558
[5]	BOSSCHE D V J, PETERS J, VERWAEREN J, et al. Mobile monitoring for mapping spatial variation in urban air quality: development and validation of a methodology based on an extensive dataset[J]. Atmospheric Environment,2015,105:148-161. doi: 10.1016/j.atmosenv.2015.01.017
[6]	WU Y Z, WANG Y X, WANG L W, et al. Application of a taxi-based mobile atmospheric monitoring system in Cangzhou, China[J]. Transportation Research Part D: Transport and Environment,2020,86:102449. doi: 10.1016/j.trd.2020.102449
[7]	RÜDIGER J, TIRPITZ J L, de MOOR J M, et al. Implementation of electrochemical, optical and denuder-based sensors and sampling techniques on UAV for volcanic gas measurements: examples from Masaya, Turrialba and Stromboli volcanoes[J]. Atmospheric Measurement Techniques,2018,11(4):2441-2457. doi: 10.5194/amt-11-2441-2018
[8]	YANG X Y, XU J, BI F, et al. Aircraft measurement over the Gulf of Tonkin capturing aloft transport of biomass burning[J]. Atmospheric Environment,2018,182:41-50. doi: 10.1016/j.atmosenv.2018.03.020
[9]	HUANG C, HU Q Y, LI Y J, et al. Intermediate volatility organic compound emissions from a large cargo vessel operated under real-world conditions[J]. Environmental Science & Technology,2018,52(21):12934-12942.
[10]	樊守彬, 杨力鹏, 程水源. 道路环境颗粒物浓度空间分布研究[J]. 环境科学与技术,2011,34(7):56-58. doi: 10.3969/j.issn.1003-6504.2011.07.015 FAN S B, YANG L P, CHENG S Y. Spatial distribution of PM₁₀ in regional road environment[J]. Environmental Science & Technology,2011,34(7):56-58. doi: 10.3969/j.issn.1003-6504.2011.07.015
[11]	贾天蛟, 葛艳丽, 刘奔, 等. 岭南亚热带森林冠层大气挥发性有机物污染特征及区域人为源的影响[J]. 环境工程技术学报,2023,13(2):473-482. JIA T J, GE Y L, LIU B, et al. Pollution characteristics of volatile organic compounds above subtropical forest canopy in Lingnan and the influence of regional anthropogenic emissions[J]. Journal of Environmental Engineering Technology,2023,13(2):473-482.
[12]	赵德龙, 周嵬, 盛久江, 等. 基于飞机观测不同天气条件下北京地区黑碳气溶胶的垂直分布及其混合态特性[J]. 环境化学,2021,40(5):1405-1412. doi: 10.1002/etc.4993 ZHAO D L, ZHOU W, SHENG J J, et al. Vertical distribution and mixed state characteristics of black carbon aerosols in Beijing Area based on aircraft observation under different weather conditions[J]. Environmental Chemistry,2021,40(5):1405-1412. doi: 10.1002/etc.4993
[13]	宋雨辰, 周胜杰, 张洪海, 等. 夏季黄海渤海上空大气颗粒物中水溶性离子浓度分布与化学特征[J]. 环境科学研究,2016,29(11):1575-1581. SONG Y C, ZHOU S J, ZHANG H H, et al. Distribution and chemical characteristics of water soluble ions in particulate matter over the Yellow Sea and the Bohai Sea in summer[J]. Research of Environmental Sciences,2016,29(11):1575-1581.
[14]	MORAWSKA L, THAI P K, LIU X T, et al. Applications of low-cost sensing technologies for air quality monitoring and exposure assessment: how far have they gone[J]. Environment International,2018,116:286-299. doi: 10.1016/j.envint.2018.04.018
[15]	李朋, 吴华成, 周卫青, 等. 民用燃煤不同燃烧阶段细颗粒物排放特征[J]. 中国环境科学,2020,40(11):4652-4659. LI P, WU H C, ZHOU W Q, et al. Emission characteristics of fine particulate matter at different combustion phases of residential coal[J]. China Environmental Science,2020,40(11):4652-4659.
[16]	RAI A C, KUMAR P, PILLA F, et al. End-user perspective of low-cost sensors for outdoor air pollution monitoring[J]. Science of the Total Environment,2017,607/608:691-705. doi: 10.1016/j.scitotenv.2017.06.266
[17]	SAYAHI T, BUTTERFIELD A, KELLY K E. Long-term field evaluation of the plantower PMS low-cost particulate matter sensors[J]. Environmental Pollution,2019,245:932-940. doi: 10.1016/j.envpol.2018.11.065
[18]	JÄRVINEN A, KUULUVAINEN H, NIEMI J V, et al. Monitoring urban air quality with a diffusion charger based electrical particle sensor[J]. Urban Climate,2015,14:441-456. doi: 10.1016/j.uclim.2014.10.002
[19]	秦孝良, 高健, 王永敏, 等. 传感器技术在环境空气监测与污染治理中的应用现状、问题与展望[J]. 中国环境监测,2019,35(4):162-172. QIN X L, GAO J, WANG Y M, et al. Application of sensor technology in environmental air monitoring and pollution control: status, problems and prospects[J]. Environmental Monitoring in China,2019,35(4):162-172.
[20]	LIU X W, XU Y S, ZENG X P, et al. Field measurements on the emission and removal of PM_2.5 from coal-fired power stations. 1: case study for a 1 000 MW ultrasupercritical utility boiler[J]. Energy & Fuels,2016,30(8):6547-6554.
[21]	汤明珍, 任建宁, 伍丽青, 等. 移动式空气质量传感器的研究与应用进展[J]. 环境科学研究,2022,35(4):971-978. TANG M Z, REN J N, WU L Q, et al. Advances in research and application of mobile air quality sensors[J]. Research of Environmental Sciences,2022,35(4):971-978.
[22]	LIN T T, LV X, HU Z N, et al. Semiconductor metal oxides as chemoresistive sensors for detecting volatile organic compounds[J]. Sensors,2019,19(2):233. doi: 10.3390/s19020233
[23]	NIKOLIC M V, MILOVANOVIC V, VASILJEVIC Z Z, et al. Semiconductor gas sensors: materials, technology, design, and application[J]. Sensors,2020,20(22):6694. doi: 10.3390/s20226694
[24]	WARDENCKI W, KATULSKI R J, STEFAŃSKI J, et al. The state of the art in the field of non-stationary instruments for the determination and monitoring of atmospheric pollutants[J]. Critical Reviews in Analytical Chemistry,2008,38(4):259-268. doi: 10.1080/10408340802378254
[25]	XIA T, CATALAN J, HU C, et al. Development of a mobile platform for monitoring gaseous, particulate, and greenhouse gas (GHG) pollutants[J]. Environmental Monitoring and Assessment,2021,193(1):7. doi: 10.1007/s10661-020-08769-2
[26]	ZHAO Y, LIU M Y. The method study on emergency detection of aromatic compounds and chlorides based on portable GC-MS[J]. Procedia Engineering,2014,84:731-735. doi: 10.1016/j.proeng.2014.10.489
[27]	KIMBROUGH S, KRABBE S, BALDAUF R, et al. The Kansas City transportation and local-scale air quality study (KC-TRAQS): integration of low-cost sensors and reference grade monitoring in a complex metropolitan area. part 1: overview of the project[J]. Chemosensors,2019,7(2):26. doi: 10.3390/chemosensors7020026
[28]	APTE J S, MESSIER K P, GANI S, et al. High-resolution air pollution mapping with google street view cars: exploiting big data[J]. Environmental Science & Technology,2017,51(12):6999-7008.
[29]	CHEN M J, YUAN W C, CAO C, et al. Development and performance evaluation of a low-cost portable PM_2.5 monitor for mobile deployment[J]. Sensors,2022,22(7):2767. doi: 10.3390/s22072767
[30]	HAGEMANN R, CORSMEIER U, KOTTMEIER C, et al. Spatial variability of particle number concentrations and NO_x in the Karlsruhe (Germany) area obtained with the mobile laboratory "AERO-TRAM"[J]. Atmospheric Environment,2014,94:341-352. doi: 10.1016/j.atmosenv.2014.05.051
[31]	ADAMS M D, DeLUCA P F, CORR D, et al. Mobile air monitoring: measuring change in air quality in the city of Hamilton, 2005-2010[J]. Social Indicators Research,2012,108(2):351-364. doi: 10.1007/s11205-012-0061-5
[32]	HASENFRATZ D, SAUKH O, WALSER C, et al. Deriving high-resolution urban air pollution maps using mobile sensor nodes[J]. Pervasive and Mobile Computing,2015,16:268-285. doi: 10.1016/j.pmcj.2014.11.008
[33]	BUKOWIECKI N, DOMMEN J, PRÉVÔT A S H, et al. A mobile pollutant measurement laboratory: measuring gas phase and aerosol ambient concentrations with high spatial and temporal resolution[J]. Atmospheric Environment,2002,36(36/37):5569-5579.
[34]	WEIJERS E P, KHLYSTOV A Y, KOS G P A, et al. Variability of particulate matter concentrations along roads and motorways determined by a moving measurement unit[J]. Atmospheric Environment,2004,38(19):2993-3002. doi: 10.1016/j.atmosenv.2004.02.045
[35]	白杨, 秦凯, 吴立新, 等. 徐州市区主干道路黑炭气溶胶浓度移动观测实验[J]. 地理与地理信息科学,2014,30(1):45-49. BAI Y, QIN K, WU L X, et al. A mobile measurement on black carbon concentrations along the main roads of Xuzhou downtown[J]. Geography and Geo-Information Science,2014,30(1):45-49.
[36]	崔爱伟, 苗纯萍, 何欢, 等. 基于移动观测的城市街道峡谷大气污染物时空分布特征[J]. 生态学杂志,2022,41(10):2035-2042. CUI A W, MIAO C P, HE H, et al. Spatiotemporal distribution characteristics of air pollutants in urban street canyons as observed by mobile monitoring[J]. Chinese Journal of Ecology,2022,41(10):2035-2042.
[37]	WALLACE J, CORR D, DELUCA P, et al. Mobile monitoring of air pollution in cities: the case of Hamilton, Ontario, Canada[J]. Journal of Environmental Monitoring,2009,11(5):998-1003. doi: 10.1039/b818477a
[38]	TARGINO A C, GIBSON M D, KRECL P, et al. Hotspots of black carbon and PM_2.5 in an urban area and relationships to traffic characteristics[J]. Environmental Pollution,2016,218:475-486. doi: 10.1016/j.envpol.2016.07.027
[39]	王红丽, 高雅琴, 景盛翱, 等. 基于走航监测的长三角工业园区周边大气挥发性有机物污染特征[J]. 环境科学,2021,42(3):1298-1305. WANG H L, GAO Y Q, JING S A, et al. Characterization of volatile organic compounds (VOCs) using mobile monitoring around the industrial parks in the yangzte river delta region of China[J]. Environmental Science,2021,42(3):1298-1305.
[40]	高家乐, 乐昊, 盖鑫磊. 南京江北化工园区挥发性有机物走航观测[J]. 环境工程,2021,39(1):89-95. GAO J L, LE H, GAI X L. Mobile measurement of ambient volatile organic compounds in the Jiangbei chemical industrial park of Nanjing, China[J]. Environmental Engineering,2021,39(1):89-95.
[41]	陈婷, 何潇, 陈文倩, 等. 基于车载测试的轻型汽车排放特征[J]. 环境工程技术学报,2022,12(4):1033-1040. CHEN T, HE X, CHEN W Q, et al. Emission characteristics of light-duty vehicles based on portable emission measurement system (PEMS)[J]. Journal of Environmental Engineering Technology,2022,12(4):1033-1040.
[42]	葛蕴珊, 丁焰, 尹航. 机动车实际行驶排放测试系统研究现状[J]. 汽车安全与节能学报,2017,8(2):111-121. doi: 10.3969/j.issn.1674-8484.2017.02.001 GE Y S, DING Y, YIN H. Research status of real driving emission measurement system for vehicles[J]. Journal of Automotive Safety and Engergy,2017,8(2):111-121. doi: 10.3969/j.issn.1674-8484.2017.02.001
[43]	KAUR S, NIEUWENHUIJSEN M J, COLVILE R N. Fine particulate matter and carbon monoxide exposure concentrations in urban street transport microenvironments[J]. Atmospheric Environment,2007,41(23):4781-4810. doi: 10.1016/j.atmosenv.2007.02.002
[44]	NAZELLE D A, FRUIN S, WESTERDAHL D, et al. A travel mode comparison of commuters' exposures to air pollutants in Barcelona[J]. Atmospheric Environment,2012,59:151-159. doi: 10.1016/j.atmosenv.2012.05.013
[45]	MINGUILLÓN M C, BRINES M, PÉREZ N, et al. New particle formation at ground level and in the vertical column over the Barcelona area[J]. Atmospheric Research,2015,164/165:118-130. doi: 10.1016/j.atmosres.2015.05.003
[46]	TANG G Q, ZHANG J Q, ZHU X W, et al. Mixing layer height and its implications for air pollution over Beijing, China[J]. Atmospheric Chemistry and Physics,2016,16(4):2459-2475. doi: 10.5194/acp-16-2459-2016
[47]	李岳, 殷宝辉, 耿春梅, 等. 武清地区冬季一次重污染过程垂直分布特征[J]. 环境科学研究,2019,32(6):1012-1019. LI Y, YIN B H, GENG C M, et al. The vertical distribution of air pollutants in a typical winter haze episode in Wuqing area[J]. Research of Environmental Sciences,2019,32(6):1012-1019.
[48]	SCHUUR E A G, McGUIRE A D, SCHÄDEL C, et al. Climate change and the permafrost carbon feedback[J]. Nature,2015,520:171-179. doi: 10.1038/nature14338
[49]	KNORR W, JIANG L, ARNETH A. Climate, CO₂ and human population impacts on global wildfire emissions[J]. Biogeosciences,2016,13(1):267-282. doi: 10.5194/bg-13-267-2016
[50]	ROBOCK A. Volcanic eruptions and climate[J]. Reviews of Geophysics,2000,38(2):191-219. doi: 10.1029/1998RG000054
[51]	PEKNEY N J, DIEHL J R, RUEHL D, et al. Measurement of methane emissions from abandoned oil and gas wells in Hillman State Park, Pennsylvania[J]. Carbon Management,2018,9(2):165-175. doi: 10.1080/17583004.2018.1443642
[52]	KOHNERT K, SERAFIMOVICH A, METZGER S, et al. Strong geologic methane emissions from discontinuous terrestrial permafrost in the Mackenzie Delta, Canada[J]. Scientific Reports,2017,7(1):1-6. doi: 10.1038/s41598-016-0028-x
[53]	OBERLE F K J, GIBBS A E, RICHMOND B M, et al. Towards determining spatial methane distribution on Arctic permafrost bluffs with an unmanned aerial system[J]. SN Applied Sciences,2019,1(3):236. doi: 10.1007/s42452-019-0242-9
[54]	AURELL J, GULLETT B, HOLDER A, et al. Wildland fire emission sampling at Fishlake National Forest, Utah using an unmanned aircraft system[J]. Atmospheric Environment,2021,247:118193. doi: 10.1016/j.atmosenv.2021.118193
[55]	SAMAD A, ALVAREZ FLOREZ D, CHOURDAKIS I, et al. Concept of using an unmanned aerial vehicle (UAV) for 3D investigation of air quality in the atmosphere: example of measurements near a roadside[J]. Atmosphere,2022,13(5):663. doi: 10.3390/atmos13050663
[56]	陈鹏飞, 张蔷, 权建农, 等. 北京地区臭氧时空分布特征的飞机探测研究[J]. 环境科学,2012,33(12):4141-4150. CHEN P F, ZHANG Q, QUAN J N, et al. Temporal and spatial distribution of ozone concentration by aircraft sounding over Beijing[J]. Chinese Journal of Environmental Science,2012,33(12):4141-4150.
[57]	刘思晗, 王红磊, 赵德龙, 等. 京津冀地区一次复合污染过程中气溶胶和BC垂直分布特征的飞机观测[J]. 地球与环境,2023,51(5):537-548. LIU S H, WANG H L, ZHAO D L, et al. Aircraft observation of aerosol and black carbon aerosol vertical distribution during a complex air pollution process in the Beijing-Tianjin-Hebei region[J]. Earth and Environment,2023,51(5):537-548.
[58]	谢文琪, 姚波, 吴国明, 等. 河北省中南部二氧化碳浓度的飞机探测研究[J]. 中国环境科学,2023,43(2):525-531. XIE W Q, YAO B, WU G M, et al. Airborne observation of carbon dioxide concentration in central and southern Hebei Province[J]. China Environmental Science,2023,43(2):525-531.
[59]	赵德龙, 肖伟, 杨燕, 等. 北京冬季重污染过程黑碳气溶胶的飞机观测[J]. 中国环境科学,2021,41(12):5539-5547. ZHAO D L, XIAO W, YANG Y, et al. Aircraft observation of black carbon aerosols during heavy pollution in winter in Beijing[J]. China Environmental Science,2021,41(12):5539-5547.
[60]	GÅLFALK M, NILSSON PÅLEDAL S, BASTVIKEN D. Sensitive drone mapping of methane emissions without the need for supplementary ground-based measurements[J]. ACS Earth and Space Chemistry,2021,5(10):2668-2676. doi: 10.1021/acsearthspacechem.1c00106
[61]	ALVARADO M, GONZALEZ F, ERSKINE P, et al. A methodology to monitor airborne PM₁₀ dust particles using a small unmanned aerial vehicle[J]. Sensors,2017,17(2):343. doi: 10.3390/s17020343
[62]	IWASZENKO S, KALISZ P, SŁOTA M, et al. Detection of natural gas leakages using a laser-based methane sensor and UAV[J]. Remote Sensing,2021,13(3):510. doi: 10.3390/rs13030510
[63]	BURGUÉS J, ESCLAPEZ M D, DOÑATE S, et al. RHINOS: a lightweight portable electronic nose for real-time odor quantification in wastewater treatment plants[J]. iScience,2021,24(12):103371. doi: 10.1016/j.isci.2021.103371
[64]	DAUGĖLA I, SUZIEDELYTE VISOCKIENE J, KUMPIENE J. Detection and analysis of methane emissions from a landfill using unmanned aerial drone systems and semiconductor sensors[J]. Detritus,2020,10:127-138.
[65]	MA J Z, WANG W, LIU H J, et al. Pollution plumes observed by aircraft over North China during the IPAC-NC field campaign[J]. Chinese Science Bulletin,2013,58(34):4329-4336. doi: 10.1007/s11434-013-5978-9
[66]	ZAVERI R A, BERKOWITZ C M, BRECHTEL F J, et al. Nighttime chemical evolution of aerosol and trace gases in a power plant plume: implications for secondary organic nitrate and organosulfate aerosol formation, NO₃ radical chemistry, and N₂O₅ heterogeneous hydrolysis[J]. Journal of Geophysical Research:Atmospheres,2010,115(D12):1-22.
[67]	ARAUJO J O, VALENTE J, KOOISTRA L, et al. Experimental flight patterns evaluation for a UAV-based air pollutant sensor[J]. Micromachines,2020,11(8):768. doi: 10.3390/mi11080768
[68]	VINKOVIĆ K, ANDERSEN T, de VRIES M, et al. Evaluating the use of an unmanned aerial vehicle (UAV)-based active AirCore system to quantify methane emissions from dairy cows[J]. Science of the Total Environment,2022,831:154898. doi: 10.1016/j.scitotenv.2022.154898
[69]	HATAKEYAMA S, MURANO K, BANDOW H, et al. The 1991 PEACAMPOT aircraft observation of ozone, NO_x, and SO₂ over the East China Sea, the Yellow Sea, and the Sea of Japan[J]. Journal of Geophysical Research:Atmospheres,1995,100(D11):23143-23151. doi: 10.1029/95JD02269
[70]	YANG X Y, JI D S, LI J W, et al. Impacts of springtime biomass burning in Southeast Asia on atmospheric carbonaceous components over the Beibu Gulf in China: insights from aircraft observations[J]. Science of the Total Environment,2023,857:159232. doi: 10.1016/j.scitotenv.2022.159232
[71]	WU H H, TAYLOR J W, SZPEK K, et al. Vertical variability of the properties of highly aged biomass burning aerosol transported over the southeast Atlantic during CLARIFY-2017[J]. Atmospheric Chemistry and Physics,2020,20(21):12697-12719. doi: 10.5194/acp-20-12697-2020
[72]	SMITH S R, ALORY G, ANDERSSON A, et al. Ship-based contributions to global ocean, weather, and climate observing systems[J]. Frontiers in Marine Science,2019,6:434. doi: 10.3389/fmars.2019.00434
[73]	WANNINKHOF R, PICKERS P A, OMAR A M, et al. A surface ocean CO₂ reference network, SOCONET and associated marine boundary layer CO₂ measurements[J]. Frontiers in Marine Science,2019,6:400. doi: 10.3389/fmars.2019.00400
[74]	CARSLAW K S, LEE L A, REDDINGTON C L, et al. Large contribution of natural aerosols to uncertainty in indirect forcing[J]. Nature,2013,503(7474):67-71. doi: 10.1038/nature12674
[75]	DUCE R A, LISS P S, MERRILL J T, et al. The atmospheric input of trace species to the world ocean[J]. Global Biogeochemical Cycles,1991,5(3):193-259. doi: 10.1029/91GB01778
[76]	SRINIVAS B, SARIN M M. Atmospheric pathways of phosphorous to the Bay of Bengal: contribution from anthropogenic sources and mineral dust[J]. Tellus Series B:Chemical and Physical Meteorology,2012,64(1):1-12.
[77]	GOLOBOKOVA L , KRUGLINSKY I , POCHUFAROV A , et al. Chemical composition of atmospheric aerosol in Arctic regions in summer 2021[J]. Izvestiya, Atmospheric and Oceanic Physics, 2023, 59(Suppl 1): S70-S80.
[78]	SUN Q B, LIANG B L, CAI M F, et al. Cruise observation of the marine atmosphere and ship emissions in South China Sea: aerosol composition, sources, and the aging process[J]. Environmental Pollution,2023,316:120539. doi: 10.1016/j.envpol.2022.120539
[79]	孔少飞, 陆炳, 韩斌, 等. 天津近海大气中CH₄, N₂O和CO₂季节变化分析[J]. 中国科学(地球科学),2010,40(5):666-676. doi: 10.1360/zd2010-40-5-666 KONG S F, LU B, HAN B, et al. Analysis of seasonal variation of CH₄, N₂O and CO₂ in Tianjin offshore atmosphere[J]. Scientia Sinica (Terrae),2010,40(5):666-676. doi: 10.1360/zd2010-40-5-666
[80]	李嘉鑫, 臧昆鹏, 林溢, 等. 海洋大气二氧化碳船基走航连续观测数据的质量控制方法[J]. 环境化学,2022,41(10):3335-3344. doi: 10.7524/j.issn.0254-6108.2021061302 LI J X, ZANG K P, LIN Y, et al. Study of data quality assurance/control on the shipborne continuous CO₂ observations[J]. Environmental Chemistry,2022,41(10):3335-3344. doi: 10.7524/j.issn.0254-6108.2021061302
[81]	盛立芳, 高会旺, 张英娟, 等. 夏季渤海NO_x、O₃、SO₂和CO浓度观测特征[J]. 环境科学,2002,23(6):31-35. SHENG L F, GAO H W, ZHANG Y J, et al. Observational characteristics of the concentrations of NO_x, O₃, SO₂ and CO over Bohai Sea in summer[J]. Chinese Journal of Environmental Science,2002,23(6):31-35.
[82]	石金辉, 张云, 高会旺, 等. 东海大气气溶胶的化学特征及来源[J]. 环境科学学报,2011,31(8):1750-1757. SHI J H, ZHANG Y, GAO H W, et al. Characteristics and sources of atmospheric aerosols over the East China Sea[J]. Acta Scientiae Circumstantiae,2011,31(8):1750-1757.
[83]	盛立芳, 郭志刚, 高会旺, 等. 渤海大气气溶胶元素组成及物源分析[J]. 中国环境监测,2005,21(1):16-21. doi: 10.3969/j.issn.1002-6002.2005.01.005 SHENG L F, GUO Z G, GAO H W, et al. Preliminary study on Element composition and source apportionment of atmospheric aerosol over Bohai Sea[J]. Environmental Monitoring in China,2005,21(1):16-21. doi: 10.3969/j.issn.1002-6002.2005.01.005
[84]	薛磊, 张洪海, 杨桂朋. 春季黄渤海大气气溶胶的离子特征与来源分析[J]. 环境科学学报,2011,31(11):2329-2335. XUE L, ZHANG H H, YANG G P. Characteristics and source analysis of atmospheric aerosol ions over the Yellow Sea and the Bohai Sea in spring[J]. Acta Scientiae Circumstantiae,2011,31(11):2329-2335.
[85]	LIANG B L, CAI M F, SUN Q B, et al. Source apportionment of marine atmospheric aerosols in northern South China Sea during summertime 2018[J]. Environmental Pollution,2021,289:117948. doi: 10.1016/j.envpol.2021.117948
[86]	YANG X Y, GAO Y G, LI Q B, et al. Maritime and coastal observations of ambient PM_2.5 and its elemental compositions in the Bohai Bay of China during spring and summer: levels, spatial distribution and source apportionment[J]. Atmospheric Research,2023,293:106897. doi: 10.1016/j.atmosres.2023.106897
[87]	付丹. 中国近海至南大洋大气NO_x及气溶胶中金属元素和PAHs分布特征及源解析[D]. 青岛: 国家海洋局第一海洋研究所, 2017.
[88]	张敏. 远洋船基及上海地基大气气溶胶理化特性研究[D]. 上海: 复旦大学, 2011.
[89]	ÜNLÜGENÇOĞLU K, KÖKKÜLÜNK G, ALARÇIN F. Estimation of shipping emissions via novel developed data collecting and calculation software: a case study for the Region of Ambarli Port[J]. International Journal of Global Warming,2019,19(3):293. doi: 10.1504/IJGW.2019.103723
[90]	EYRING V, KÖHLER H W, van AARDENNE J, et al. Emissions from international shipping: 1. the last 50 years[J]. Journal of Geophysical Research:Atmospheres,2005,110(D17):1-12.
[91]	BAI C J, LI Y, LIU B X, et al. Gaseous emissions from a seagoing ship under different operating conditions in the coastal region of China[J]. Atmosphere,2020,11(3):305. doi: 10.3390/atmos11030305
[92]	WINNES H, FRIDELL E. Emissions of NO_x and particles from manoeuvring ships[J]. Transportation Research Part D:Transport and Environment,2010,15(4):204-211. doi: 10.1016/j.trd.2010.02.003
[93]	COOPER D A. Exhaust emissions from ships at berth[J]. Atmospheric Environment,2003,37(27):3817-3830. doi: 10.1016/S1352-2310(03)00446-1
[94]	van CHU T, RISTOVSKI Z, POURKHESALIAN M A, et al. On-board measurements of particle and gaseous emissions from a large cargo vessel at different operating conditions[J]. Environmental Pollution,2018,237:832-841. doi: 10.1016/j.envpol.2017.11.008
[95]	WINNES H, FRIDELL E. Particle emissions from ships: dependence on fuel type[J]. Journal of the Air & Waste Management Association,2009,59(12):1391-1398.
[96]	WINNES H, MOLDANOVÁ J, ANDERSON M, et al. On-board measurements of particle emissions from marine engines using fuels with different sulphur content[J]. Proceedings of the Institution of Mechanical Engineers, Part M: Journal of Engineering for the Maritime Environment, 2016, 230(1): 45-54.
[97]	FU M L, DING Y, GE Y S, et al. Real-world emissions of inland ships on the Grand Canal, China[J]. Atmospheric Environment,2013,81:222-229. □ doi: 10.1016/j.atmosenv.2013.08.046