Study on the distribution characteristics of air particle concentration in urban agglomeration in China
-
摘要:
利用2015—2022年颗粒物(PM2.5和PM10)监测数据,从浓度水平和统计学分布2个角度,采用日均浓度、年均浓度、概率论角度达标情况和达标所需浓度降低量4个维度分析我国10个城市群(169个城市)的颗粒物浓度分布特征及异同。结果表明,我国城市群内部颗粒物浓度污染水平趋于平稳,城市群之间颗粒物浓度差异较大。我国城市群颗粒物浓度存在分层现象,根据颗粒物浓度水平将10个城市群分为高浓度、中浓度、低浓度城市群3类。从统计学分布角度也分为3类,但关中平原城市群被划分到高浓度城市群,其余城市群分类则不变。我国城市群之间颗粒物达标( GB 3095—2012《环境空气质量标准》二级标准)所需浓度降低量差异显著。海峡西岸城市群的PM2.5和PM10以及珠三角城市群的PM10已经达标,而中原、关中平原、京津冀和山东半岛城市群如果要达标,PM2.5和PM10浓度分别需降低50%和27%以上。建议科学制定符合我国国情的颗粒物区域阶段目标值,推动城市群结合自身情况加快分阶段达标。
Abstract:Based on the monitoring data of particulate matter (PM2.5 and PM10) from 2015 to 2022, the concentration distribution characteristics and similarities and differences of particulate matter in 10 urban agglomerations (169 cities) in China were analyzed from the perspectives of daily average concentration, annual average concentration, compliance from a probability theory angle, and the required concentration reduction for compliance. The results indicated that the pollution levels of particulate matter within urban agglomerations in China tend to stabilize, while significant differences existed among different urban agglomerations. The concentration of particulate matter within urban agglomerations in China exhibited a stratified pattern. Based on the concentration levels, the 10 urban agglomerations were categorized into three groups: high, medium, and low concentrations. This classification remained consistent when viewed from a statistical distribution perspective, except for the Guanzhong Plain urban agglomeration, which was classified as a high-concentration urban agglomeration. The differences in the required concentration reduction for compliance (secondary standard of Ambient Air Quality Standard (GB 3095-2012)) were significant among urban agglomerations. The PM2.5 and PM10 levels in the Western Taiwan Strait urban agglomerations and the PM10 levels in the Pearl River Delta urban agglomeration have already met the standards. However, in order for the Central Plains, Guanzhong Plain, Beijing-Tianjin-Hebei, and Shandong Peninsula urban agglomerations to meet the standards, the concentration of PM2.5 and PM10 needed to be reduced by more than 50% and 27%, respectively. It was recommended to scientifically establish regional stage target values for particulate matter in line with China's national conditions, to accelerate compliance in urban agglomerations in stages based on their own conditions.s.
-
表 1 10个城市群PM2.5和PM10未达标频率
Table 1. Frequency of PM2.5 and PM10 non-compliance in 10 urban agglomerations
% 城市群 PM2.5 PM10 ZY 13.7 7.3 GZPY 11.0 6.9 JJJ 7.9 3.5 SDBD 6.6 3.1 CY 5.7 1.1 CJZY 4.7 0.8 LZN 3.1 0.8 CSJ 1.8 0.4 ZSJ 0.5 0.0 HXXA 0.1 0.0 表 2 10个城市群PM2.5和PM10超标临界浓度及达标所需降低量
Table 2. Exceeding critical concentration and reduction required for PM2.5 and PM10 compliance in 10 urban agglomerations
城市群 PM2.5 PM10 超标临界浓度/
(μg/m3)降低量/% 超标临界浓度/
(μg/m3)降低量/% ZY 205.70 63.5 287.41 47.8 GZPY 189.89 60.5 294.19 49.0 JJJ 177.64 57.8 240.07 37.5 SDBD 158.96 52.8 206.53 27.4 CY 150.04 50.0 192.23 22.0 CJZY 139.12 46.1 177.26 15.4 LZN 125.60 40.3 178.24 15.8 CSJ 106.32 29.5 157.56 4.8 ZSJ 85.51 12.3 103.40 −45.1 HXXA 63.56 −18.0 86.60 −73.2 -
[1] 阚海东, 陈秉衡, 汪宏. 上海市城区大气颗粒物污染对居民健康危害的经济学评价[J]. 中国卫生经济,2004,23(2):8-11. doi: 10.3969/j.issn.1003-0743.2004.02.003 [2] 穆泉, 张世秋. 中国2001—2013年PM2.5重污染的历史变化与健康影响的经济损失评估[J]. 北京大学学报(自然科学版),2015,51(4):694-706.MU Q, ZHANG S Q. Assessment of the trend of heavy PM2.5 pollution days and economic loss of health effects during 2001-2013[J]. Acta Scientiarum Naturalium Universitatis Pekinensis,2015,51(4):694-706. [3] 刘爱明, 杨柳, 吴亚玲, 等. 城市区域大气颗粒物的健康效应研究[J]. 中国环境监测,2012,28(5):19-23. doi: 10.3969/j.issn.1002-6002.2012.05.005LIU A M, YANG L, WU Y L, et al. Research on the health effects of atmospheric particulates in city region[J]. Environmental Monitoring in China,2012,28(5):19-23. doi: 10.3969/j.issn.1002-6002.2012.05.005 [4] 张晓平, 张燕萍, 封宝琴, 等. 太原市大气可吸入颗粒物对心脑血管疾病死亡的影响[J]. 疾病监测,2007,22(8):556-559. doi: 10.3784/j.issn.1003-9961.2007.08.019ZHANG X P, ZHANG Y P, FENG B Q, et al. Effects of PM10 on the mortality of cerebrocardiovascular diseases in Taiyuan[J]. Disease Surveillance,2007,22(8):556-559. doi: 10.3784/j.issn.1003-9961.2007.08.019 [5] 陈卫红, 曹丽敏, 刘跃伟, 等. 空气细颗粒物与呼吸系统的健康损害[J]. 公共卫生与预防医学,2016,27(3):1-4.CHEN W H, CAO L M, LIU Y W, et al. The adverse health effects of atmosphere fine particulate matter on respiratory system[J]. Journal of Public Health and Preventive Medicine,2016,27(3):1-4. [6] 陈仁杰, 陈秉衡, 阚海东. 我国113个城市大气颗粒物污染的健康经济学评价[J]. 中国环境科学,2010,30(3):410-415.CHEN R J, CHEN B H, KAN H D. A health-based economic assessment of particulate air pollution in 113 Chinese Cities[J]. China Environmental Science,2010,30(3):410-415. [7] COHEN A J, BRAUER M, BURNETT R, et al. Estimates and 25-year trends of the global burden of disease attributable to ambient air pollution: an analysis of data from the Global Burden of Diseases Study 2015[J]. The Lancet,2017,389:1907-1918. doi: 10.1016/S0140-6736(17)30505-6 [8] CHRISTOPHER P, MURRAY J L. Global burden of 87 risk factors in 204 countries and territories, 1990-2019: a systematic analysis for the Global Burden of Disease Study 2019[J]. The Lancet,2020,396:1223-1249. doi: 10.1016/S0140-6736(20)30752-2 [9] SALTZMAN B E. Health risk assessment of fluctuating concentrations using lognormal models[J]. Journal of the Air & Waste Management Association,1997,47(11):1152-1160. [10] FANG C L, LIU H M, LI G D. International progress and evaluation on interactive coupling effects between urbanization and the eco-environment[J]. Journal of Geographical Sciences,2016,26(8):1081-1116. doi: 10.1007/s11442-016-1317-9 [11] 刘艳菊, 杨峥, 刘庆阳, 等. 北京4个功能区春冬季大气重污染期间PM10和PM2.5化学污染特征及影响因素分析[J]. 环境工程技术学报,2021,11(4):631-646. doi: 10.12153/j.issn.1674-991X.20200214LIU Y J, YANG Z, LIU Q Y, et al. Chemical pollution characteristic of PM10 and PM2.5 during heavy air pollution in spring and winter in four functional areas of Beijing and their associated influencing factors[J]. Journal of Environmental Engineering Technology,2021,11(4):631-646. doi: 10.12153/j.issn.1674-991X.20200214 [12] 江家坤, 马莹, 黄学良, 等. 云浮市2018—2020年颗粒物和臭氧污染特征及污染案例研究[J]. 环境科学研究,2022,35(3):691-698.JIANG J K, MA Y, HUANG X L, et al. Pollution characteristics and a pollution case of particulate matter and O3 in Yunfu City from 2018 to 2020[J]. Research of Environmental Sciences,2022,35(3):691-698. [13] 杨玖, 代佼, 龚兴涛, 等. 攀枝花市大气污染物特征及气象因子关系分析[J]. 环境科学与技术,2022,45(增刊1):205-214.YANG J, DAI J, GONG X T, et al. Characteristics of atmospheric pollutants and correlation analysis of meteorological parameters in Panzhihua[J]. Environmental Science & Technology,2022,45(Suppl 1):205-214. [14] 赵丽多, 任丽红, 李军, 等. 云南省芒市春季PM2.5水溶性离子特征及来源分析[J]. 环境工程技术学报,2021,11(6):1057-1064. doi: 10.12153/j.issn.1674-991X.20210073ZHAO L D, REN L H, LI J, et al. Characteristics and source analysis of water-soluble ions of PM2.5 during spring in Mang City, Yunnan Province[J]. Journal of Environmental Engineering Technology,2021,11(6):1057-1064. doi: 10.12153/j.issn.1674-991X.20210073 [15] 史军, 崔林丽. 长江三角洲城市群霾的演变特征及影响因素研究[J]. 中国环境科学,2013,33(12):2113-2122.SHI J, CUI L L. Characteristics and influencing factors of haze in the Yangtze River Delta region[J]. China Environmental Science,2013,33(12):2113-2122. [16] 李明珠, 徐峻, 刘厚凤, 等. 济南都市圈PM2.5来源贡献分析[J]. 环境工程技术学报,2021,11(2):209-216. doi: 10.12153/j.issn.1674-991X.20200145LI M Z, XU J, LIU H F, et al. PM2.5 source apportionment over Jinan Metropolitan Area[J]. Journal of Environmental Engineering Technology,2021,11(2):209-216. doi: 10.12153/j.issn.1674-991X.20200145 [17] 刘海猛, 方创琳, 黄解军, 等. 京津冀城市群大气污染的时空特征与影响因素解析[J]. 地理学报,2018,73(1):177-191. doi: 10.11821/dlxb201801015LIU H M, FANG C L, HUANG J J, et al. The spatial-temporal characteristics and influencing factors of air pollution in Beijing-Tianjin-Hebei urban agglomeration[J]. Acta Geographica Sinica,2018,73(1):177-191. doi: 10.11821/dlxb201801015 [18] 李雁宇, 李杰, 曾胜兰, 等. 2017年汾渭平原东部大气颗粒物污染特征分析[J]. 环境科学研究,2020,33(1):63-72.LI Y Y, LI J, ZENG S L, et al. Analysis of atmospheric particulates in the eastern Fenwei plain in 2017[J]. Research of Environmental Sciences,2020,33(1):63-72. [19] 崔宏, 刘肖, 秦巧燕. 汾渭平原典型污染城市PM2.5来源分布及传输分析[J]. 环境工程技术学报,2022,12(5):1593-1600.CUI H, LIU X, QIN Q Y. PM2.5 source distribution and transmission analysis in typical polluted cities of Fenwei Plain[J]. Journal of Environmental Engineering Technology,2022,12(5):1593-1600. [20] 杨欣, 何友江, 廉涵阳, 等. 天山北坡区域大气污染特征及冬季重污染成因分析: 以石河子市为例[J]. 环境工程技术学报,2023,13(2):483-490.YANG X, HE Y J, LIAN H Y, et al. Characteristics of the air pollution and the causes of heavy air pollution in winter in the northern slope of Tianshan Mountains: case study of Shihezi City[J]. Journal of Environmental Engineering Technology,2023,13(2):483-490. [21] 郭一鸣, 蔺雪芹, 边宇. 中国城市群空气质量时空演化特征及其影响因素[J]. 生态经济,2019(11):167-175.GUO Y M, LIN X Q, BIAN Y. The spatial-temporal characteristics and influencing factors of air quality in China’s urban agglomerations[J]. Ecological Economy,2019(11):167-175. [22] 王振波, 梁龙武, 王旭静. 中国城市群地区PM2.5时空演变格局及其影响因素[J]. 地理学报,2019,74(12):2614-2630. doi: 10.11821/dlxb201912014WANG Z B, LIANG L W, WANG X J. Spatio-temporal evolution patterns and influencing factors of PM2.5 in Chinese urban agglomerations[J]. Acta Geographica Sinica,2019,74(12):2614-2630. doi: 10.11821/dlxb201912014 [23] 万庆, 罗翔, 潘方杰, 等. 中国城市群空气质量时空演化及收敛趋势[J]. 地理科学,2022,42(11):1943-1953.WAN Q, LUO X, PAN F J, et al. Spatial-temporal evolution and convergence trend of air quality in China’s urban agglomerations[J]. Scientia Geographica Sinica,2022,42(11):1943-1953. [24] GEORGOPOULOS P G, SEINFELD J H. Statistical distributions of air pollutant concentrations[J]. Environmental Science & Technology,1982,16(7):401-416. [25] KAO A S, FRIEDLANDER S K. Frequency distributions of PM10 chemical components and their sources[J]. Environmental Science & Technology,1995,29(1):19-28. [26] MARANI A, LAVAGNINI I, BUTTAZZONI C. Statistical study of air pollutant concentrations via generalized gamma distributions[J]. Journal of the Air Pollution Control Association,1986,36(11):1250-1254. doi: 10.1080/00022470.1986.10466173 [27] MOREL B, YEH S, CIFUENTES L. Statistical distributions for air pollution applied to the study of the particulate problem in Santiago[J]. Atmospheric Environment,1999,33(16):2575-2585. doi: 10.1016/S1352-2310(98)00380-X [28] KARACA F, ALAGHA O, ERTÜRK F. Statistical characterization of atmospheric PM10 and PM2.5 concentrations at a non-impacted suburban site of Istanbul, Turkey[J]. Chemosphere,2005,59(8):1183-1190. doi: 10.1016/j.chemosphere.2004.11.062 [29] LU H C. The statistical characters of PM10 concentration in Taiwan area[J]. Atmospheric Environment,2002,36(3):491-502. doi: 10.1016/S1352-2310(01)00245-X [30] DONG K. Statistical distributions of ambient air pollutants in Shanghai, China[J]. Biomedical and Environmental Sciences,2004,17(3):366-372. [31] WANG X, CHEN R J, CHEN B H, et al. Application of statistical distribution of PM10 concentration in air quality management in 5 representative cities of China[J]. Biomedical and Environmental Sciences,2013,26(8):638-646. [32] 李晶, 钱妮生, 修光利. 大气污染物小时浓度统计分布方法及其应用[J]. 环境科学与技术,2015,38(11):82-87.LI J, QIAN N S, XIU G L. Statistical distribution of air pollutant hourly average concentrations: method and its application[J]. Environmental Science & Technology,2015,38(11):82-87. [33] JIANG X, DENG S X, LIU N, et al. The statistical distributions of SO2, NO2 and PM10 concentrations in Xi'an, China[C]//2011 International Symposium on Water Resource and Environmental Protection. Xi'an: IEEE, 2011: 2206-2212. [34] 邓启红, 黄柏良, 唐猛, 等. 长沙市大气颗粒物PM10质量浓度的统计分布特性[J]. 中南大学学报(自然科学版),2012,43(4):1567-1573.DENG Q H, HUANG B L, TANG M, et al. Statistical distributions of PM10 during summer in Changsha, China[J]. Journal of Central South University,2012,43(4):1567-1573. [35] 曹艳, 彭秀云, 孟静. 呼包鄂城市群PM2.5质量浓度统计分布特性[J]. 数学的实践与认识,2019,49(10):244-253.CAO Y, PENG X Y, MENG J. Statistical characteristics of PM2.5 concentration in Hohhot-Baotou-Ordos region[J]. Mathematics in Practice and Theory,2019,49(10):244-253. [36] SAMOLI E, ANALITIS A, TOULOUMI G, et al. Estimating the exposure-response relationships between particulate matter and mortality within the APHEA multicity project[J]. Environmental Health Perspectives,2005,113(1):88-95. doi: 10.1289/ehp.7387 [37] ABBEY D, NISHINO N, MCDONNELL W, et al. Long-term inhalable particles and other air pollutants related to mortality in nonsmokers[J]. American Journal of Respiratory and Critical Care Medicine,1999,159(2):373-382. doi: 10.1164/ajrccm.159.2.9806020 [38] 中华人民共和国国民经济和社会发展第十三个五年规划纲要[A/OL]. (2016-03-17)[2023-08-15]. https://www.gov.cn/xinwen/2016-03/17/content_5054992.htm. [39] 郭锐, 孙勇, 樊杰. “十四五” 时期中国城市群 分类治理的政策[J]. 中国科学院院刊,2020,35(7):844-854.GUO R, SUN Y, FAN J. Policies on categorized governance of China's urban agglomerations in 14th Five-Year plan[J]. Bulletin of the Chinese Academy of Sciences,2020,35(7):844-854. [40] 中国环境监测总站. 全国城市空气质量实时发布平台[EB/OL]. [2023-08-15]. http://ifgga3e1da9b3884544c3svq6qq5of5wpn6pk9.fhaz.libproxy.ruc.edu.cn/. [41] 环境保护部. 环境空气质量标准:GB 3095—2012[S]. 北京: 中国环境科学出版社, 2012. [42] 环境保护部. 环境空气质量评价技术规范(试行):HJ 663—2013 [S]. 北京: 中国环境科学出版社, 2013. [43] 生态环境部. 受沙尘天气过程影响城市空气质量评价补充规定[A/OL]. (2017-01-04)[2023-12-07]. https://www.mee.gov.cn/gkml/hbb/bgt/201701/t20170106_394054.htm. [44] 山东省生态环境厅. 山东省大气污染防治条例[A/OL]. (2016-07-26)[2023-11-11]. http://sthj.shandong.gov.cn/dtxx/hbyw/201607/t20160726_774112.html. [45] 山东省生态环境厅. 山东省环境保护厅关于印发进一步加强省会城市群大气污染防治工作实施方案的通知[A/OL]. (2016-10-09)[2023-11-11]. http://xxgk.sdein.gov.cn/zfwj/lhf/201610/t20161009_1172654.html. [46] 北京市生态环境局. 京津冀三地环保厅局签署区域环境保护率先突破合作框架协议[A/OL]. (2015-12-04)[2023-11-11]. https://sthjj.beijing.gov.cn/bjhrb/index/xxgk69/sthjlyzwg/wrygl/602670/index.html. [47] 生态环境部. 关于印发《京津冀及周边地区2017—2018年秋冬季大气污染综合治理攻坚行动方案》的通知[A/OL]. (2017-08-21)[2023-11-11]. https://www.mee.gov.cn/gkml/hbb/bwj/201708/t20170824_420330.htm. [48] 国家发展和改革委员会. 关中平原城市群发展规划[A/OL]. (2018-02-07)[2023-08-15]. https://www.ndrc.gov.cn/xxgk/zcfb/ghwb/201802/t20180207_962246.html. □